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Effect of Metal Ion Intercalation on the Structure of MXene and Water Dynamics on its Internal Surfaces
Open accessAbstract
MXenes are a recently discovered class of 2D materials with an excellent potential for energy storage applications. Because MXene surfaces are hydrophilic and attractive interaction forces between the layers are relatively weak, water molecules can spontaneously intercalate at ambient humidity and significantly influence the key properties of this 2D material. Using complementary X-ray and neutron scattering techniques, we demonstrate that intercalation with potassium cations significantly improves structural homogeneity and water stability in MXenes. In agreement with molecular dynamics simulations, intercalated potassium ions reduce the water self-diffusion coefficient by 2 orders of magnitude, suggesting greater stability of hydrated MXene against changing environmental conditions.
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Cited by
Antioxidants Unlock Shelf-Stable Ti3C2T (MXene) Nanosheet Dispersions
Zhao, X., Vashisth, A., Prehn, E., Sun, W., Shah, S. A., Habib, T., Chen, Y., Tan, Z., Lutkenhaus, J. L., Radovic, M., et al. (2019) · Matter · doi:10.1016/j.matt.2019.05.020 · Cited by 747
A Review on MXene Synthesis, Stability, and Photocatalytic Applications
Murali, G., Reddy Modigunta, J. K., Park, Y. H., Lee, J.-H., Rawal, J., Lee, S.-Y., In, I., & Park, S.-J. (2022) · ACS Nano · doi:10.1021/acsnano.2c04750 · Cited by 668
Recent Advances in Oxidation Stable Chemistry of 2D MXenes
Cao, F., Zhang, Y., Wang, H., Khan, K., Tareen, A. K., Qian, W., Zhang, H., & Ågren, H. (2022) · Advanced Materials · doi:10.1002/adma.202107554 · Cited by 648
Two-Dimensional Ti3C2Tx MXene Nanosheets for Efficient Copper Removal from Water
Shahzad, A., Rasool, K., Miran, W., Nawaz, M., Jang, J., Mahmoud, K. A., & Lee, D. S. (2017) · ACS Sustainable Chemistry & Engineering · doi:10.1021/acssuschemeng.7b02695 · Cited by 478
Ti3C2 2D MXene: Recent Progress and Perspectives in Photocatalysis
Tang, R., Xiong, S., Gong, D., Deng, Y., Wang, Y., Su, L., Ding, C., Yang, L., & Liao, C. (2020) · ACS Applied Materials & Interfaces · doi:10.1021/acsami.0c12905 · Cited by 259
Metadata
- Authors
- Osti, N. C., Naguib, M., Ostadhossein, A., Xie, Y., Kent, P. R. C., Dyatkin, B., Rother, G., Heller, W. T., van Duin, A. C. T., Gogotsi, Y., & Mamontov, E.
- Venue
- ACS Applied Materials & Interfaces
- Publisher
- American Chemical Society (ACS)
- Published
- 2016-03-30
- Volume
- 8
- Issue
- 14
- Pages
- 8859-8863
- ISSN
- 1944-8244 (ISSN-L)
- 1944-8252
- OpenAlex
- W2306697644
- Cited by
- 315
- References
- 0
- FWCI
- 10.91
- Type
- journal article
- Language
- en
- Open access
- green
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- Osti, N. C., Naguib, M., Ostadhossein, A., Xie, Y., Kent, P. R. C., Dyatkin, B., Rother, G., Heller, W. T., van Duin, A. C. T., Gogotsi, Y., & Mamontov, E. (2016). Effect of Metal Ion Intercalation on the Structure of MXene and Water Dynamics on its Internal Surfaces. ACS Applied Materials & Interfaces. https://doi.org/10.1021/acsami.6b01490
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