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Toward Inexpensive Photocatalytic Hydrogen Evolution: A Nickel Sulfide Catalyst Supported on a High-Stability Metal–Organic Framework
Open accessAbstract
Few-atom clusters composed of nickel and sulfur have been successfully installed into the Zr(IV)-based metal-organic framework (MOF) NU-1000 via ALD-like chemistry (ALD = atomic layer deposition). X-ray photoelectron spectroscopy and Raman spectroscopy are used to determine that primarily Ni(2+) and S(2-) sites are deposited within the MOF. In a pH 7 buffered aqueous solution, the porous catalyst is able to produce H2 gas at a rate of 3.1 mmol g(-1) h(-1) upon UV irradiation, whereas no H2 is generated by irradiating bare NU-1000. Upon visible light irradiation, little H2 generation was observed; however, with the addition of an organic dye, rose bengal, NiS-AIM can catalyze the production of H2 at an enhanced rate of 4.8 mmol g(-1) h(-1). These results indicate that ALD in MOFs (AIM) can engender reactivity within high surface area supports for applications in the solar fuels field.
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Cites
Biomimetic Hydrogen Evolution: MoS 2 Nanoparticles as Catalyst for Hydrogen Evolution
Hinnemann, B., Moses, P. G., Bonde, J., Jørgensen, K. P., Nielsen, J. H., Horch, S., Chorkendorff, I., & Nørskov, J. K. (2005) · Journal of the American Chemical Society · doi:10.1021/ja0504690 · Cited by 4,065
Roles of Cocatalysts in Photocatalysis and Photoelectrocatalysis
Yang, J., Wang, D., Han, H., & Li, C. (2013) · Accounts of Chemical Research · doi:10.1021/ar300227e · Cited by 2,848
Horike, S., Shimomura, S., & Kitagawa, S. (2009) · Nature Chemistry · doi:10.1038/nchem.444 · Cited by 2,486
Nanostructured hydrotreating catalysts for electrochemical hydrogen evolution
Morales-Guio, C. G., Stern, L.-A., & Hu, X. (2014) · Chemical Society Reviews · doi:10.1039/c3cs60468c · Cited by 2,437
Gao, M.-R., Xu, Y.-F., Jiang, J., & Yu, S.-H. (2013) · Chemical Society Reviews · doi:10.1039/c2cs35310e · Cited by 1,610
Yan, Y., Xia, B., Xu, Z., & Wang, X. (2014) · ACS Catalysis · doi:10.1021/cs500070x · Cited by 868
Hod, I., Deria, P., Bury, W., Mondloch, J. E., Kung, C.-W., So, M., Sampson, M. D., Peters, A. W., Kubiak, C. P., Farha, O. K., et al. (2015) · Nature Communications · doi:10.1038/ncomms9304 · Cited by 290
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Ma, X., Liu, H., Yang, W., Mao, G., Zheng, L., & Jiang, H.-L. (2021) · Journal of the American Chemical Society · doi:10.1021/jacs.1c05032 · Cited by 445
Das, S., Ghosh, R., Routh, P., Shit, A., Mondal, S., Panja, A., & Nandi, A. K. (2018) · ACS Applied Nano Materials · doi:10.1021/acsanm.8b00373 · Cited by 59
Metadata
- Authors
- Peters, A. W., Li, Z., Farha, O. K., & Hupp, J. T.
- Venue
- ACS Applied Materials & Interfaces
- Publisher
- American Chemical Society (ACS)
- Published
- 2016-08-03
- Volume
- 8
- Issue
- 32
- Pages
- 20675-20681
- ISSN
- 1944-8244 (ISSN-L)
- 1944-8252
- OpenAlex
- W2506894030
- Cited by
- 182
- References
- 7
- FWCI
- 6.70
- Type
- journal article
- Language
- en
- Open access
- green
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