The DOI matches its Crossref record; 2 of the 2 references it cites were found in a registry or an index.
Purification of Perovskite Quantum Dots Using Low-Dielectric-Constant Washing Solvent “Diglyme” for Highly Efficient Light-Emitting Devices
Abstract
Cesium lead halide (CsPbX 3, X = Cl, Br, or I) perovskite quantum dots (QDs) are known as ionic nanocrystals, and their optical properties are greatly affected by the washing solvent used during the purification process. Here, we demonstrate the purification process of CsPbBr 3 perovskite QDs using low-dielectric-constant solvents to completely remove impurities, such as the reaction solvent and desorbed ligands. The use of the ether solvent diethylene glycol dimethyl ether (diglyme), having a low dielectric constant of ε = 7.23, as a poor solvent for reprecipitation allowed for multiple wash cycles, which led to high purity and high photoluminescence quantum yield for CsPbBr 3 QDs. The light-emitting device constructed with the CsPbBr 3 QDs and washed twice with diglyme (two-wash) showed a low turn-on voltage of 2.7 V and a peak external quantum efficiency of over 8%. Thus, the purification of perovskite QDs with multiple wash cycles using a low-dielectric-constant solvent is an effective approach for enhancing not only the optical properties but also the efficiency of perovskite quantum dot light-emitting devices.
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Cites
Akkerman, Q. A., D’Innocenzo, V., Accornero, S., Scarpellini, A., Petrozza, A., Prato, M., & Manna, L. (2015) · Journal of the American Chemical Society · doi:10.1021/jacs.5b05602 · Cited by 2,197
Vashishtha, P., & Halpert, J. E. (2017) · Chemistry of Materials · doi:10.1021/acs.chemmater.7b01609 · Cited by 353
Cited by
Wei, Y., Cheng, Z., & Lin, J. (2019) · Chemical Society Reviews · doi:10.1039/c8cs00740c · Cited by 1,206
Metal Halide Perovskite Light‐Emitting Devices: Promising Technology for Next‐Generation Displays
Lu, M., Zhang, Y., Wang, S., Guo, J., Yu, W. W., & Rogach, A. L. (2019) · Advanced Functional Materials · doi:10.1002/adfm.201902008 · Cited by 425
Surface Chemistry Engineering of Perovskite Quantum Dots: Strategies, Applications, and Perspectives
Bai, Y., Hao, M., Ding, S., Chen, P., & Wang, L. (2022) · Advanced Materials · doi:10.1002/adma.202105958 · Cited by 394
Blue perovskite light-emitting diodes: progress, challenges and future directions
Kumawat, N. K., Liu, X.-K., Kabra, D., & Gao, F. (2019) · Nanoscale · doi:10.1039/c8nr09885a · Cited by 268
Metadata
- Authors
- Hoshi, K., Chiba, T., Sato, J., Hayashi, Y., Takahashi, Y., Ebe, H., Ohisa, S., & Kido, J.
- Venue
- ACS Applied Materials & Interfaces
- Publisher
- American Chemical Society (ACS)
- Published
- 2018-07-03
- Volume
- 10
- Issue
- 29
- Pages
- 24607-24612
- ISSN
- 1944-8244 (ISSN-L)
- 1944-8252
- OpenAlex
- W2810006447
- Cited by
- 161
- References
- 2
- FWCI
- 6.02
- Type
- journal article
- Language
- en
- Open access
- closed
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