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Cerium-Oxide-Modified Nickel as a Non-Noble Metal Catalyst for Selective Decomposition of Hydrous Hydrazine to Hydrogen
Abstract
Hydrous hydrazine is identified as a hydrogen reservoir owing to its high content of hydrogen (8.0 wt %). Its selective decomposition under mild conditions is the key for quick H 2 release. Modifying Ni nanoparticles with a small amount of CeO 2 (8.0 mol %) resulted in a 3-fold increase of turnover frequency (TOF) and an enhancement of H 2 selectivity from 67% to above 99%. This improvement was due to the modification of Ni with CeO 2 nearby through strong metal–support interaction (e.g., Ni–O–Ce structure). Furthermore, this promoting effect was extended to other oxides which can form strong metal–support interaction with Ni, such as ZrO 2, MgO, and La 2 O 3 .
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Bruix, A., Rodriguez, J. A., Ramírez, P. J., Senanayake, S. D., Evans, J., Park, J. B., Stacchiola, D., Liu, P., Hrbek, J., & Illas, F. (2012) · Journal of the American Chemical Society · doi:10.1021/ja302070k · Cited by 839
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The recent development of efficient Earth-abundant transition-metal nanocatalysts
Wang, D., & Astruc, D. (2017) · Chemical Society Reviews · doi:10.1039/c6cs00629a · Cited by 608
Zhou, P., Hai, G., Zhao, G., Li, R., Huang, X., Lu, Y., & Wang, G. (2023) · Applied Catalysis B: Environmental · doi:10.1016/j.apcatb.2023.122364 · Cited by 259
Akbayrak, S., Tonbul, Y., & Özkar, S. (2017) · Applied Catalysis B: Environmental · doi:10.1016/j.apcatb.2017.01.063 · Cited by 134
Metadata
- Authors
- He, L., Liang, B., Li, L., Yang, X., Huang, Y., Wang, A., Wang, X., & Zhang, T.
- Venue
- ACS Catalysis
- Publisher
- American Chemical Society (ACS)
- Published
- 2015-02-11
- Volume
- 5
- Issue
- 3
- Pages
- 1623-1628
- ISSN
- 2155-5435 (ISSN-L)
- OpenAlex
- W2330278132
- Cited by
- 159
- References
- 1
- FWCI
- 7.86
- Type
- journal article
- Language
- en
- Open access
- closed
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- He, L., Liang, B., Li, L., Yang, X., Huang, Y., Wang, A., Wang, X., & Zhang, T. (2015). Cerium-Oxide-Modified Nickel as a Non-Noble Metal Catalyst for Selective Decomposition of Hydrous Hydrazine to Hydrogen. ACS Catalysis. https://doi.org/10.1021/acscatal.5b00143
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