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High Activity Oxygen Evolution Reaction Catalysts from Additive-Controlled Electrodeposited Ni and NiFe Films
Abstract
Electrodeposition of Ni or NiFe films exhibiting fractal-like behavior from plating baths containing an inhibitor, such as 3,5-diamino-1,2,4-triazole (DAT), is found to yield oxygen evolution reaction (OER) catalysts for alkaline solutions exhibiting high current densities (100 mA/cm 2 ), high mass activity (∼1200 A/g of catalyst), high stability (>72 h), and low overpotentials (∼300 mV). By changing electrodeposition time, the activity of the catalyst can be tuned, with longer times yielding higher activities. The electrodeposition method works with any conductive substrate yielding unprecedented performance and providing an easy route to high activity catalysts.
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Cites
Hunter, B. M., Blakemore, J. D., Deimund, M., Gray, H. B., Winkler, J. R., & Müller, A. M. (2014) · Journal of the American Chemical Society · doi:10.1021/ja506087h · Cited by 321
Cited by
Hoang, T. T. H., Verma, S., Ma, S., Fister, T. T., Timoshenko, J., Frenkel, A. I., Kenis, P. J. A., & Gewirth, A. A. (2018) · Journal of the American Chemical Society · doi:10.1021/jacs.8b01868 · Cited by 852
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Browne, M. P., Sofer, Z., & Pumera, M. (2019) · Energy & Environmental Science · doi:10.1039/c8ee02495b · Cited by 396
Qiu, Z., Ma, Y., & Edvinsson, T. (2019) · Nano Energy · doi:10.1016/j.nanoen.2019.104118 · Cited by 382
Intralayered Ostwald Ripening to Ultrathin Nanomesh Catalyst with Robust Oxygen‐Evolving Performance
Xie, J., Zhang, X., Zhang, H., Zhang, J., Li, S., Wang, R., Pan, B., & Xie, Y. (2017) · Advanced Materials · doi:10.1002/adma.201604765 · Cited by 339
Nanoporous Copper Films by Additive-Controlled Electrodeposition: CO2 Reduction Catalysis
Hoang, T. T. H., Ma, S., Gold, J. I., Kenis, P. J. A., & Gewirth, A. A. (2017) · ACS Catalysis · doi:10.1021/acscatal.6b03613 · Cited by 296
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Metadata
- Authors
- Hoang, T. T. H., & Gewirth, A. A.
- Venue
- ACS Catalysis
- Publisher
- American Chemical Society (ACS)
- Published
- 2016-01-20
- Volume
- 6
- Issue
- 2
- Pages
- 1159-1164
- ISSN
- 2155-5435 (ISSN-L)
- OpenAlex
- W2255802039
- Cited by
- 171
- References
- 1
- FWCI
- 7.14
- Type
- journal article
- Language
- en
- Open access
- closed
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- Hoang, T. T. H., & Gewirth, A. A. (2016). High Activity Oxygen Evolution Reaction Catalysts from Additive-Controlled Electrodeposited Ni and NiFe Films. ACS Catalysis. https://doi.org/10.1021/acscatal.5b02365
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