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Tri-s-triazine-Based Crystalline Graphitic Carbon Nitrides for Highly Efficient Hydrogen Evolution Photocatalysis
Abstract
Graphitic carbon nitride (g-CN) is an emerging metal-free photocatalyst for solar energy conversion via water splitting and CO 2 fixation. Herein, we used preheated melamine as a starting material in combination with the salt melt method to synthesize a crystalline tri- s -triazine-based g-CN. The as-obtained sample exhibited high stability and photocatalytic activity toward hydrogen and oxygen production from water splitting. In addition, by adding phosphate to mimic natural photosynthetic environment, the apparent quantum yield (AQY) for the hydrogen production reached 50.7% at 405 nm, which is the highest value ever reported for conjugated carbon nitride polymers in hydrogen evolution photocatalysis. The results of this study demonstrate that crystalline covalent tri- s -triazine frameworks hold great promise for solar energy applications.
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Cited by
Xu, Q., Zhu, B., Jiang, C., Cheng, B., & Yu, J. (2018) · Solar RRL · doi:10.1002/solr.201800006 · Cited by 486
Enhanced Photocatalytic H2O2 Production over Carbon Nitride by Doping and Defect Engineering
Wu, S., Yu, H., Chen, S., & Quan, X. (2020) · ACS Catalysis · doi:10.1021/acscatal.0c03359 · Cited by 466
Zhang, G., Lan, Z.-A., & Wang, X. (2017) · Chemical Science · doi:10.1039/c7sc01747b · Cited by 357
Self-citationFull‐Spectrum Solar‐Light‐Activated Photocatalysts for Light–Chemical Energy Conversion
Wang, X., Wang, F., Sang, Y., & Liu, H. (2017) · Advanced Energy Materials · doi:10.1002/aenm.201700473 · Cited by 328
Self-citationLin, L., Ren, W., Wang, C., Asiri, A. M., Zhang, J., & Wang, X. (2018) · Applied Catalysis B: Environmental · doi:10.1016/j.apcatb.2018.03.009 · Cited by 312
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Metadata
- Authors
- Lin, L., Ou, H., Zhang, Y., & Wang, X.
- Venue
- ACS Catalysis
- Publisher
- American Chemical Society (ACS)
- Published
- 2016-05-20
- Volume
- 6
- Issue
- 6
- Pages
- 3921-3931
- ISSN
- 2155-5435 (ISSN-L)
- OpenAlex
- W2385556747
- Cited by
- 950
- References
- 6
- FWCI
- 24.85
- Type
- journal article
- Language
- en
- Open access
- closed
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