The DOI matches its Crossref record; 65 of the 65 references it cites were found in a registry or an index.
Catalytic Advantages, Challenges, and Priorities in Alkaline Membrane Fuel Cells
Abstract
Recently, anion exchange membrane fuel cells (AEMFCs) have seen a significant growth in research and practical interest as the achievable current density, peak power density, and longevity of state-of-the-art cells have improved dramatically. Though these advances in performance have been important for demonstrating the feasibility of the technology, nearly all AEMFCs reported in the literature have required a relatively high loading of platinum group metal (PGM)-based catalysts at both the anode and cathode electrode to achieve even adequate, let alone exemplary, performance. However, in order to take command of the low-temperature fuel cell market, AEMFCs cannot simply reach the same performance as incumbent proton exchange membrane fuel cells (PEMFCs), which have had decades of development and investment. AEMFCs must be able to realize their most widely quoted advantage over PEMFCs and be produced at a much lower cost than PEMFCs. In the long run, the most likely pathway to acceptably low cost AEMFCs will involve the deployment of PGM-free catalysts at both electrodes. In this Viewpoint, we will discuss what we believe are the most promising approaches to achieve PGM-free catalysts for the oxygen reduction reaction (AEMFC cathode) and hydrogen oxidation reaction (AEMFC anode), as well as provide our perspective on key issues that must be addressed to craft these catalysts into high-performing, durable electrodes.
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Cites
Anion-exchange membranes in electrochemical energy systems
Varcoe, J. R., Atanassov, P., Dekel, D. R., Herring, A. M., Hickner, M. A., Kohl, P. A., Kucernak, A. R., Mustain, W. E., Nijmeijer, K., Scott, K., et al. (2014) · Energy Environ. Sci. · doi:10.1039/c4ee01303d · Cited by 2,051
Self-citationHydrogen Oxidation and Evolution Reaction Kinetics on Platinum: Acid vs Alkaline Electrolytes
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Direct atomic-level insight into the active sites of a high-performance PGM-free ORR catalyst
Chung, H. T., Cullen, D. A., Higgins, D., Sneed, B. T., Holby, E. F., More, K. L., & Zelenay, P. (2017) · Science · doi:10.1126/science.aan2255 · Cited by 1,684
New insights into the electrochemical hydrogen oxidation and evolution reaction mechanism
Durst, J., Siebel, A., Simon, C., Hasché, F., Herranz, J., & Gasteiger, H. A. (2014) · Energy Environ. Sci. · doi:10.1039/c4ee00440j · Cited by 1,666
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Iron-based cathode catalyst with enhanced power density in polymer electrolyte membrane fuel cells
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Oxygen Reduction in Alkaline Media: From Mechanisms to Recent Advances of Catalysts
Ge, X., Sumboja, A., Wuu, D., An, T., Li, B., Goh, F. W. T., Hor, T. S. A., Zong, Y., & Liu, Z. (2015) · ACS Catalysis · doi:10.1021/acscatal.5b00524 · Cited by 1,341
A review of Fe–N/C and Co–N/C catalysts for the oxygen reduction reaction
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Review of cell performance in anion exchange membrane fuel cells
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Poly(aryl piperidinium) membranes and ionomers for hydroxide exchange membrane fuel cells
Wang, J., Zhao, Y., Setzler, B. P., Rojas-Carbonell, S., Ben Yehuda, C., Amel, A., Page, M., Wang, L., Hu, K., Shi, L., et al. (2019) · Nature Energy · doi:10.1038/s41560-019-0372-8 · Cited by 1,012
Cited by
Xiao, F., Wang, Y., Wu, Z., Chen, G., Yang, F., Zhu, S., Siddharth, K., Kong, Z., Lu, A., Li, J., et al. (2021) · Advanced Materials · doi:10.1002/adma.202006292 · Cited by 614
Zhang, B., Wang, J., Liu, G., Weiss, C. M., Liu, D., Chen, Y., Xia, L., Zhou, P., Gao, M., Liu, Y., et al. (2024) · Nature Catalysis · doi:10.1038/s41929-024-01126-3 · Cited by 567
Single-Atom (Iron-Based) Catalysts: Synthesis and Applications
Singh, B., Gawande, M. B., Kute, A. D., Varma, R. S., Fornasiero, P., McNeice, P., Jagadeesh, R. V., Beller, M., & Zbořil, R. (2021) · Chemical Reviews · doi:10.1021/acs.chemrev.1c00158 · Cited by 373
Alloying Nickel with Molybdenum Significantly Accelerates Alkaline Hydrogen Electrocatalysis
Wang, M., Yang, H., Shi, J., Chen, Y., Zhou, Y., Wang, L., Di, S., Zhao, X., Zhong, J., Cheng, T., et al. (2021) · Angewandte Chemie International Edition · doi:10.1002/anie.202013047 · Cited by 285
Zhao, G., Jiang, Y., Dou, S.-X., Sun, W., & Pan, H. (2021) · Science Bulletin · doi:10.1016/j.scib.2020.09.014 · Cited by 253
Metadata
- Authors
- Firouzjaie, H. A., & Mustain, W. E.
- Venue
- ACS Catalysis
- Publisher
- American Chemical Society (ACS)
- Published
- 2019-11-21
- Volume
- 10
- Issue
- 1
- Pages
- 225-234
- ISSN
- 2155-5435 (ISSN-L)
- OpenAlex
- W2989990727
- Cited by
- 313
- References
- 65
- Type
- journal article
- Language
- en
- Open access
- closed
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