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Synthesis of Single Atom Based Heterogeneous Platinum Catalysts: High Selectivity and Activity for Hydrosilylation Reactions
Open accessAbstract
High Resolution Image Download MS PowerPoint Slide Catalytic hydrosilylation represents a straightforward and atom-efficient methodology for the creation of C–Si bonds. In general, the application of homogeneous platinum complexes prevails in industry and academia. Herein, we describe the first heterogeneous single atom catalysts (SACs), which are conveniently prepared by decorating alumina nanorods with platinum atoms. The resulting stable material efficiently catalyzes hydrosilylation of industrially relevant olefins with high TON (≈10 5 ). A variety of substrates is selectively hydrosilylated including compounds with sensitive reducible and other functional groups (N, B, F, Cl). The single atom based catalyst shows significantly higher activity compared to related Pt nanoparticles.
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Citations
Cites
Catalysis by Supported Single Metal Atoms
Liu, J. (2017) · ACS Catalysis · doi:10.1021/acscatal.6b01534 · Cited by 1,331
Cited by
Sarma, B. B., Maurer, F., Doronkin, D. E., & Grunwaldt, J.-D. (2023) · Chemical Reviews · doi:10.1021/acs.chemrev.2c00495 · Cited by 291
Metadata
- Authors
- Cui, X., Junge, K., Dai, X., Kreyenschulte, C., Pohl, M.-M., Wohlrab, S., Shi, F., Brückner, A., & Beller, M.
- Venue
- ACS Central Science
- Publisher
- American Chemical Society (ACS)
- Published
- 2017-05-17
- Volume
- 3
- Issue
- 6
- Pages
- 580-585
- ISSN
- 2374-7943 (ISSN-L)
- 2374-7951
- OpenAlex
- W2616545756
- Cited by
- 163
- References
- 1
- FWCI
- 7.19
- Type
- journal article
- Language
- en
- Open access
- diamond
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- The paper
- Cui, X., Junge, K., Dai, X., Kreyenschulte, C., Pohl, M.-M., Wohlrab, S., Shi, F., Brückner, A., & Beller, M. (2017). Synthesis of Single Atom Based Heterogeneous Platinum Catalysts: High Selectivity and Activity for Hydrosilylation Reactions. ACS Central Science. https://doi.org/10.1021/acscentsci.7b00105
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