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Bifunctional Surface Engineering on SnO2 Reduces Energy Loss in Perovskite Solar Cells
Open accessAbstract
Tin oxide (SnO 2 ) has recently emerged as a promising electron transport layer for perovskite solar cells (PSCs) in light of the material’s optical and electronic properties and its low-temperature processing. However, SnO 2 films are prone to surface defect formation, which results in energy loss in PSCs. We report that surface treatment using ammonium fluoride (NH 4 F) leads to reduced surface defects and that it also induces chemical doping of the SnO 2 substrate simultaneously. The effects of NH 4 F treatment on SnO 2 properties are revealed by surface chemical analysis, computational studies, and energy level investigations, and PSCs with the treatment achieve photovoltaic performance of 23.2% in light of higher voltage than in relevant controls.
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Cites
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Cited by
Recent progress in perovskite solar cells: from device to commercialization
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Metadata
- Authors
- Jung, E. H., Chen, B., Bertens, K., Vafaie, M., Teale, S., Proppe, A., Hou, Y., Zhu, T., Zheng, C., & Sargent, E. H.
- Venue
- ACS Energy Letters
- Publisher
- American Chemical Society (ACS)
- Published
- 2020-08-04
- Volume
- 5
- Issue
- 9
- Pages
- 2796-2801
- ISSN
- 2380-8195 (ISSN-L)
- OpenAlex
- W3047518622
- Cited by
- 389
- References
- 17
- FWCI
- 18.57
- Type
- journal article
- Language
- en
- Open access
- green
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- Jung, E. H., Chen, B., Bertens, K., Vafaie, M., Teale, S., Proppe, A., Hou, Y., Zhu, T., Zheng, C., & Sargent, E. H. (2020). Bifunctional Surface Engineering on SnO2 Reduces Energy Loss in Perovskite Solar Cells. ACS Energy Letters. https://doi.org/10.1021/acsenergylett.0c01566
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