The DOI matches its Crossref record; 27 of the 27 references it cites were found in a registry or an index.
Aqueous Mg-Ion Battery Based on Polyimide Anode and Prussian Blue Cathode
Abstract
The magnesium-metal battery, which consists of a cathode, a Mg-metal anode, and a nonaqueous electrolyte, is a safer and less expensive alternative to the popular Li-ion battery. However, the performance of Mg batteries is greatly limited by the low electrochemical oxidative stability of nonaqueous electrolytes, the slow Mg 2+ diffusion into the cathode, and the irreversibility of Mg striping and plating on the Mg metal anode. Here, we report the first Mg-ion battery using a Mg 2+ aqueous electrolyte, nickel hexacyanoferrate cathode, and polyimide anode. The operation depends on Mg 2+ intercalation–deintercalation at the cathode and reversible enolization at the anode, accompanied by Mg 2+ transport between cathode and anode. The cell exhibits a maximum cell voltage of 1.5 V and a supercapacitor-like high power, and it can be cycled 5000 times. This system points the way to improved Mg-based rechargeable batteries.
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Cites
Where do batteries end and supercapacitors begin?
Simon, P., Gogotsi, Y., & Dunn, B. (2014) · Science · doi:10.1126/science.1249625 · Cited by 5,634
Prototype systems for rechargeable magnesium batteries
Aurbach, D., Lu, Z., Schechter, A., Gofer, Y., Gizbar, H., Turgeman, R., Cohen, Y., Moshkovich, M., & Levi, E. (2000) · Nature · doi:10.1038/35037553 · Cited by 2,355
A metal-free organic–inorganic aqueous flow battery
Huskinson, B., Marshak, M. P., Suh, C., Er, S., Gerhardt, M. R., Galvin, C. J., Chen, X., Aspuru-Guzik, A., Gordon, R. G., & Aziz, M. J. (2014) · Nature · doi:10.1038/nature12909 · Cited by 1,585
Aqueous Rechargeable Li and Na Ion Batteries
Kim, H., Hong, J., Park, K.-Y., Kim, H., Kim, S.-W., & Kang, K. (2014) · Chemical Reviews · doi:10.1021/cr500232y · Cited by 1,493
Mg rechargeable batteries: an on-going challenge
Yoo, H. D., Shterenberg, I., Gofer, Y., Gershinsky, G., Pour, N., & Aurbach, D. (2013) · Energy & Environmental Science · doi:10.1039/c3ee40871j · Cited by 1,398
Nickel Hexacyanoferrate Nanoparticle Electrodes For Aqueous Sodium and Potassium Ion Batteries
Wessells, C. D., Peddada, S. V., Huggins, R. A., & Cui, Y. (2011) · Nano Letters · doi:10.1021/nl203193q · Cited by 1,074
Luo, J.-Y., Cui, W.-J., He, P., & Xia, Y.-Y. (2010) · Nature Chemistry · doi:10.1038/nchem.763 · Cited by 948
Self-citationPolyimides: Promising Energy‐Storage Materials
Song, Z., Zhan, H., & Zhou, Y. (2010) · Angewandte Chemie International Edition · doi:10.1002/anie.201002439 · Cited by 713
Electrolyte roadblocks to a magnesium rechargeable battery
Muldoon, J., Bucur, C. B., Oliver, A. G., Sugimoto, T., Matsui, M., Kim, H. S., Allred, G. D., Zajicek, J., & Kotani, Y. (2012) · Energy & Environmental Science · doi:10.1039/c2ee03029b · Cited by 667
Rechargeable magnesium battery: Current status and key challenges for the future
Saha, P., Datta, M. K., Velikokhatnyi, O. I., Manivannan, A., Alman, D., & Kumta, P. N. (2014) · Progress in Materials Science · doi:10.1016/j.pmatsci.2014.04.001 · Cited by 649
Cited by
Rechargeable Aqueous Zn–V2O5 Battery with High Energy Density and Long Cycle Life
Zhang, N., Dong, Y., Jia, M., Bian, X., Wang, Y., Qiu, M., Xu, J., Liu, Y., Jiao, L., & Cheng, F. (2018) · ACS Energy Letters · doi:10.1021/acsenergylett.8b00565 · Cited by 1,052
Self-citationOpportunities and Challenges for Organic Electrodes in Electrochemical Energy Storage
Poizot, P., Gaubicher, J., Renault, S., Dubois, L., Liang, Y., & Yao, Y. (2020) · Chemical Reviews · doi:10.1021/acs.chemrev.9b00482 · Cited by 963
Prussian Blue Cathode Materials for Sodium‐Ion Batteries and Other Ion Batteries
Qian, J., Wu, C., Cao, Y., Ma, Z., Huang, Y., Ai, X., & Yang, H. (2018) · Advanced Energy Materials · doi:10.1002/aenm.201702619 · Cited by 871
Voltage issue of aqueous rechargeable metal-ion batteries
Liu, Z., Huang, Y., Huang, Y., Yang, Q., Li, X., Huang, Z., & Zhi, C. (2020) · Chemical Society Reviews · doi:10.1039/c9cs00131j · Cited by 783
Prussian Blue Analogs for Rechargeable Batteries
Wang, B., Han, Y., Wang, X., Bahlawane, N., Pan, H., Yan, M., & Jiang, Y. (2018) · iScience · doi:10.1016/j.isci.2018.04.008 · Cited by 499
Metadata
- Authors
- Chen, L., Bao, J. L., Dong, X., Truhlar, D. G., Wang, Y., Wang, C., & Xia, Y.
- Venue
- ACS Energy Letters
- Publisher
- American Chemical Society (ACS)
- Published
- 2017-04-21
- Volume
- 2
- Issue
- 5
- Pages
- 1115-1121
- ISSN
- 2380-8195 (ISSN-L)
- OpenAlex
- W2606029598
- Cited by
- 369
- References
- 27
- FWCI
- 13.76
- Type
- journal article
- Language
- en
- Open access
- closed
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- Chen, L., Bao, J. L., Dong, X., Truhlar, D. G., Wang, Y., Wang, C., & Xia, Y. (2017). Aqueous Mg-Ion Battery Based on Polyimide Anode and Prussian Blue Cathode. ACS Energy Letters. https://doi.org/10.1021/acsenergylett.7b00040
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