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Orientation-Dependent Oxygen Evolution on RuO2 without Lattice Exchange
Open accessAbstract
RuO 2 catalysts exhibit record activities toward the oxygen evolution reaction (OER), which is crucial to enable efficient and sustainable energy storage. Here we examine the RuO 2 OER kinetics on rutile (110), (100), (101), and (111) orientations, finding (100) the most active. We assess the potential involvement of lattice oxygen in the OER mechanism with online electrochemical mass spectrometry, which showed no evidence of oxygen exchange on these oriented facets in acidic or basic electrolytes. Similar results were obtained for polyoriented RuO 2 films and particles, in contrast to previous work, suggesting lattice oxygen is not exchanged in catalyzing OER on crystalline RuO 2 surfaces. This hypothesis is supported by the correlation of activity with the number of active Ru-sites calculated by density functional theory, where more active facets bind oxygen more weakly. This new understanding of the active sites provides a design strategy to enhance the OER activity of RuO 2 nanoparticles by facet engineering.
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Universality in Oxygen Evolution Electrocatalysis on Oxide Surfaces
Man, I. C., Su, H., Calle‐Vallejo, F., Hansen, H. A., Martínez, J. I., Inoglu, N. G., Kitchin, J., Jaramillo, T. F., Nørskov, J. K., & Rossmeisl, J. (2011) · ChemCatChem · doi:10.1002/cctc.201000397 · Cited by 4,769
Self-citationReier, T., Nong, H. N., Teschner, D., Schlögl, R., & Strasser, P. (2017) · Advanced Energy Materials · doi:10.1002/aenm.201601275 · Cited by 1,253
Cited by
A review on fundamentals for designing oxygen evolution electrocatalysts
Song, J., Wei, C., Huang, Z.-F., Liu, C., Zeng, L., Wang, X., & Xu, Z. J. (2020) · Chemical Society Reviews · doi:10.1039/c9cs00607a · Cited by 2,936
Self-citationChatenet, M., Pollet, B. G., Dekel, D. R., Dionigi, F., Deseure, J., Millet, P., Braatz, R. D., Bazant, M. Z., Eikerling, M., Staffell, I., et al. (2022) · Chemical Society Reviews · doi:10.1039/d0cs01079k · Cited by 2,025
Self-citationChen, F.-Y., Wu, Z.-Y., Adler, Z., & Wang, H. (2021) · Joule · doi:10.1016/j.joule.2021.05.005 · Cited by 1,284
Wu, Z.-Y., Chen, F.-Y., Li, B., Yu, S.-W., Finfrock, Y. Z., Meira, D. M., Yan, Q.-Q., Zhu, P., Chen, M.-X., Song, T.-W., et al. (2023) · Nature Materials · doi:10.1038/s41563-022-01380-5 · Cited by 1,004
Lin, Y., Tian, Z., Zhang, L., Ma, J., Jiang, Z., Deibert, B. J., Ge, R., & Chen, L. (2019) · Nature Communications · doi:10.1038/s41467-018-08144-3 · Cited by 734
Metadata
- Authors
- Stoerzinger, K. A., Diaz-Morales, O., Kolb, M., Rao, R. R., Frydendal, R., Qiao, L., Wang, X. R., Halck, N. B., Rossmeisl, J., Hansen, H. A., Vegge, T., Stephens, I. E. L., Koper, M. T. M., & Shao-Horn, Y.
- Venue
- ACS Energy Letters
- Publisher
- American Chemical Society (ACS)
- Published
- 2017-03-20
- Volume
- 2
- Issue
- 4
- Pages
- 876-881
- ISSN
- 2380-8195 (ISSN-L)
- OpenAlex
- W2597898713
- Cited by
- 387
- References
- 2
- FWCI
- 7.40
- Type
- journal article
- Language
- en
- Open access
- green
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- Stoerzinger, K. A., Diaz-Morales, O., Kolb, M., Rao, R. R., Frydendal, R., Qiao, L., Wang, X. R., Halck, N. B., Rossmeisl, J., Hansen, H. A., Vegge, T., Stephens, I. E. L., Koper, M. T. M., & Shao-Horn, Y. (2017). Orientation-Dependent Oxygen Evolution on RuO2 without Lattice Exchange. ACS Energy Letters. https://doi.org/10.1021/acsenergylett.7b00135
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