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Fluorescent Alloy CsPbxMn1–xI3 Perovskite Nanocrystals with High Structural and Optical Stability
Open accessAbstract
Abstract CsPbI3 nanocrystals are still limited in their use because of their phase instability as they degrade into the yellow nonemitting δ-CsPbI3 phase within a few days. We show that alloyed CsPbxMn1–xI3 nanocrystals have essentially the same optical features and crystal structure as the parent α-CsPbI3 system, but they are stable in films and in solution for periods over a month. The stabilization stems from a small decrease in the lattice parameters slightly increasing the Goldsmith tolerance factor, combined with an increase in the cohesive energy. Finally, hybrid density functional calculations confirm that the Mn2+ levels fall within the conduction band, thus not strongly altering the optical properties.
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Cites
Strongly emissive perovskite nanocrystal inks for high-voltage solar cells
Akkerman, Q. A., Gandini, M., Di Stasio, F., Rastogi, P., Palazon, F., Bertoni, G., Ball, J. M., Prato, M., Petrozza, A., & Manna, L. (2016) · Nature Energy · doi:10.1038/nenergy.2016.194 · Cited by 721
Self-citation
Cited by
Genesis, challenges and opportunities for colloidal lead halide perovskite nanocrystals
Akkerman, Q. A., Rainò, G., Kovalenko, M. V., & Manna, L. (2018) · Nature Materials · doi:10.1038/s41563-018-0018-4 · Cited by 2,287
Self-citationWei, Y., Cheng, Z., & Lin, J. (2019) · Chemical Society Reviews · doi:10.1039/c8cs00740c · Cited by 1,206
Metal-Doped Lead Halide Perovskites: Synthesis, Properties, and Optoelectronic Applications
Zhou, Y., Chen, J., Bakr, O. M., & Sun, H.-T. (2018) · Chemistry of Materials · doi:10.1021/acs.chemmater.8b02989 · Cited by 650
Swarnkar, A., Mir, W. J., & Nag, A. (2018) · ACS Energy Letters · doi:10.1021/acsenergylett.7b01197 · Cited by 554
Mn2+‐Doped Metal Halide Perovskites: Structure, Photoluminescence, and Application
Su, B., Zhou, G., Huang, J., Song, E., Nag, A., & Xia, Z. (2021) · Laser & Photonics Reviews · doi:10.1002/lpor.202000334 · Cited by 319
Metadata
- Authors
- Akkerman, Q. A., Meggiolaro, D., Dang, Z., De Angelis, F., & Manna, L.
- Venue
- ACS Energy Letters
- Publisher
- American Chemical Society (ACS)
- Published
- 2017-08-31
- Volume
- 2
- Issue
- 9
- Pages
- 2183-2186
- ISSN
- 2380-8195 (ISSN-L)
- OpenAlex
- W2746192832
- Cited by
- 368
- References
- 1
- FWCI
- 17.45
- Type
- journal article
- Language
- en
- Open access
- hybrid
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- Akkerman, Q. A., Meggiolaro, D., Dang, Z., De Angelis, F., & Manna, L. (2017). Fluorescent Alloy CsPbxMn1–xI3 Perovskite Nanocrystals with High Structural and Optical Stability. ACS Energy Letters. https://doi.org/10.1021/acsenergylett.7b00707
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