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Guided Lithium Metal Deposition and Improved Lithium Coulombic Efficiency through Synergistic Effects of LiAsF6 and Cyclic Carbonate Additives
Abstract
Spatial and morphology control over lithium (Li) metal nucleation and growth, as well as improving Li Coulombic efficiency (CE), are among the most challenging issues for rechargeable Li metal batteries. Here, we report that LiAsF 6 and cyclic carbonate additives such as vinylene carbonate (VC) or fluoroethylene carbonate (FEC) can work synergistically to address these challenges. It is revealed that LiAsF 6 can be reduced to Li x As alloy and LiF, which act as nanosized seeds for Li growth and form a robust solid electrolyte interface layer. The addition of VC or FEC not only enables the uniform distribution of Li x As seeds but also improves the flexibility of the solid electrolyte interface layer. As a result, highly compact, uniform, and dendrite-free Li film with vertically aligned column structure can be obtained with increased Li CE, and the Li metal batteries using the electrolyte with both LiAsF 6 and cyclic carbonate additives can have improved cycle life.
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Michan, A. L., Parimalam, B. S., Leskes, M., Kerber, R. N., Yoon, T., Grey, C. P., & Lucht, B. L. (2016) · Chemistry of Materials · doi:10.1021/acs.chemmater.6b02282 · Cited by 541
Cited by
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Self-citationAdvancing Lithium Metal Batteries
Liu, B., Zhang, J.-G., & Xu, W. (2018) · Joule · doi:10.1016/j.joule.2018.03.008 · Cited by 1,647
Self-citationZhang, H., Eshetu, G. G., Judez, X., Li, C., Rodriguez‐Martínez, L. M., & Armand, M. (2018) · Angewandte Chemie International Edition · doi:10.1002/anie.201712702 · Cited by 774
Strategies towards enabling lithium metal in batteries: interphases and electrodes
Horstmann, B., Shi, J., Amine, R., Werres, M., He, X., Jia, H., Hausen, F., Cekic-Laskovic, I., Wiemers-Meyer, S., Lopez, J., et al. (2021) · Energy & Environmental Science · doi:10.1039/d1ee00767j · Cited by 298
Self-citationExploring the Impact of Mechanical Pressure on the Performance of Anode-Free Lithium Metal Cells
Louli, A. J., Genovese, M., Weber, R., Hames, S. G., Logan, E. R., & Dahn, J. R. (2019) · Journal of The Electrochemical Society · doi:10.1149/2.0091908jes · Cited by 282
Metadata
- Authors
- Ren, X., Zhang, Y., Engelhard, M. H., Li, Q., Zhang, J.-G., & Xu, W.
- Venue
- ACS Energy Letters
- Publisher
- American Chemical Society (ACS)
- Published
- 2017-11-17
- Volume
- 3
- Issue
- 1
- Pages
- 14-19
- ISSN
- 2380-8195 (ISSN-L)
- OpenAlex
- W2768460422
- Cited by
- 194
- References
- 1
- FWCI
- 10.29
- Type
- journal article
- Language
- en
- Open access
- closed
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- Ren, X., Zhang, Y., Engelhard, M. H., Li, Q., Zhang, J.-G., & Xu, W. (2018). Guided Lithium Metal Deposition and Improved Lithium Coulombic Efficiency through Synergistic Effects of LiAsF6 and Cyclic Carbonate Additives. ACS Energy Letters. https://doi.org/10.1021/acsenergylett.7b00982
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