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Aqueous Magnesium Zinc Hybrid Battery: An Advanced High-Voltage and High-Energy MgMn2O4 Cathode
Abstract
Driven by energy demand and commercial necessities, rechargeable aqueous metal ion batteries (RAMBs) have gained increasing attention over the last few decades as high-power and high-energy hubs for large-scale and ecofriendly energy storage devices (ESDs). However, recently explored RAMBs still do not provide the performance needed in order to be realized in grid-scale storage operations due to their poor electrochemical stability, low capacity, low working voltage, and apparently low specific energies. Herein, we have fabricated a new RAMB using MgMn 2 O 4 as the cathode and zinc as the anode for the first time. The stable electrochemical performance of this RAMB at high current rates (∼80% capacity retention at 500 mA g –1 after 500 cycles) and a very high specific energy of 370 Wh kg –1 at a specific power of 70 W kg –1 make this newcomer to the family of RAMBs a serious contender for the exploration of safe and green ESDs in the near future.
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Cited by
Voltage issue of aqueous rechargeable metal-ion batteries
Liu, Z., Huang, Y., Huang, Y., Yang, Q., Li, X., Huang, Z., & Zhi, C. (2020) · Chemical Society Reviews · doi:10.1039/c9cs00131j · Cited by 783
Alleviation of Dendrite Formation on Zinc Anodes via Electrolyte Additives
Guo, X., Zhang, Z., Li, J., Luo, N., Chai, G.-L., Miller, T. S., Lai, F., Shearing, P., Brett, D. J. L., Han, D., et al. (2021) · ACS Energy Letters · doi:10.1021/acsenergylett.0c02371 · Cited by 594
Advances and Perspectives of Cathode Storage Chemistry in Aqueous Zinc-Ion Batteries
Wang, X., Zhang, Z., Xi, B., Chen, W., Jia, Y., Feng, J., & Xiong, S. (2021) · ACS Nano · doi:10.1021/acsnano.1c01389 · Cited by 531
An Overview and Future Perspectives of Rechargeable Zinc Batteries
Shi, Y., Chen, Y., Shi, L., Wang, K., Wang, B., Li, L., Ma, Y., Li, Y., Sun, Z., Ali, W., et al. (2020) · Small · doi:10.1002/smll.202000730 · Cited by 389
Eutectic electrolyte based on N-methylacetamide for highly reversible zinc–iodine battery
Yang, Y., Liang, S., Lu, B., & Zhou, J. (2022) · Energy & Environmental Science · doi:10.1039/d1ee03268b · Cited by 285
Metadata
- Authors
- Soundharrajan, V., Sambandam, B., Kim, S., Mathew, V., Jo, J., Kim, S., Lee, J., Islam, S., Kim, K., Sun, Y.-K., & Kim, J.
- Venue
- ACS Energy Letters
- Publisher
- American Chemical Society (ACS)
- Published
- 2018-07-20
- Volume
- 3
- Issue
- 8
- Pages
- 1998-2004
- ISSN
- 2380-8195 (ISSN-L)
- OpenAlex
- W2883356219
- Cited by
- 216
- References
- 0
- FWCI
- 9.13
- Type
- journal article
- Language
- en
- Open access
- closed
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- CoChat. (2026). Citation check: Aqueous Magnesium Zinc Hybrid Battery: An Advanced High-Voltage and High-Energy MgMn2O4 Cathode. https://app.cochat.ai/papers/10.1021/acsenergylett.8b01105
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- Soundharrajan, V., Sambandam, B., Kim, S., Mathew, V., Jo, J., Kim, S., Lee, J., Islam, S., Kim, K., Sun, Y.-K., & Kim, J. (2018). Aqueous Magnesium Zinc Hybrid Battery: An Advanced High-Voltage and High-Energy MgMn2O4 Cathode. ACS Energy Letters. https://doi.org/10.1021/acsenergylett.8b01105
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