The DOI matches its Crossref record; 36 of the 36 references it cites were found in a registry or an index.
Roll-to-Roll Printing of Perovskite Solar Cells
Abstract
High efficiency combined with transformative roll-to-roll (R2R) printability makes metal halide perovskite-based solar cells the most promising solar technology to address the terawatt challenge of the future energy demand. However, translation from lab-scale deposition solution processing techniques to large-scale R2R methods has typically led to reduced photovoltaic performance. Here, we demonstrate large-scale, highly crystalline, uniaxially oriented, smooth perovskite films printed at room temperature and in the ambient environment. Confirmed with high speed in situ X-ray diffraction measurements, the perovskite films reach 98% of relative crystallinity at room temperature and display high texture within 1 s of the coating. We demonstrate an all-blade-coated metal halide perovskite cell with power conversion efficiency (PCE) up to 19.6%, a slot-die coated cell with a PCE of 17.3%, and a partially R2R slot-die coated flexible glass-based cell efficiency of 14.1%. The developed printing method can be applied to diverse perovskite compositions, enabling a variety of bandgaps to pave the way for the future R2R printing of highly efficient perovskite–perovskite tandem cells.
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Cites
Solvent engineering for high-performance inorganic–organic hybrid perovskite solar cells
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Compositional engineering of perovskite materials for high-performance solar cells
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Fabrication and processing of polymer solar cells: A review of printing and coating techniques
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National Renewable Energy Laboratory
Karim, S., Faissal, A., & Noureddine, E. B. (2022) · Handbook of Algal Biofuels · doi:10.1016/b978-0-12-823764-9.00006-6 · Cited by 2,558
Promises and challenges of perovskite solar cells
Correa-Baena, J.-P., Saliba, M., Buonassisi, T., Grätzel, M., Abate, A., Tress, W., & Hagfeldt, A. (2017) · Science · doi:10.1126/science.aam6323 · Cited by 2,221
A vacuum flash–assisted solution process for high-efficiency large-area perovskite solar cells
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Perovskite-perovskite tandem photovoltaics with optimized band gaps
Eperon, G. E., Leijtens, T., Bush, K. A., Prasanna, R., Green, T., Wang, J. T.-W., McMeekin, D. P., Volonakis, G., Milot, R. L., May, R., et al. (2016) · Science · doi:10.1126/science.aaf9717 · Cited by 1,499
Scalable fabrication of perovskite solar cells
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Self-citationToward Large Scale Roll‐to‐Roll Production of Fully Printed Perovskite Solar Cells
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Cited by
Tin Oxide Electron‐Selective Layers for Efficient, Stable, and Scalable Perovskite Solar Cells
Altinkaya, C., Aydin, E., Ugur, E., Isikgor, F. H., Subbiah, A. S., De Bastiani, M., Liu, J., Babayigit, A., Allen, T. G., Laquai, F., et al. (2021) · Advanced Materials · doi:10.1002/adma.202005504 · Cited by 348
Kim, Y. Y., Yang, T.-Y., Suhonen, R., Kemppainen, A., Hwang, K., Jeon, N. J., & Seo, J. (2020) · Nature Communications · doi:10.1038/s41467-020-18940-5 · Cited by 319
Iodine reduction for reproducible and high-performance perovskite solar cells and modules
Chen, S., Xiao, X., Gu, H., & Huang, J. (2021) · Science Advances · doi:10.1126/sciadv.abe8130 · Cited by 312
Local Crystal Misorientation Influences Non-radiative Recombination in Halide Perovskites
Jariwala, S., Sun, H., Adhyaksa, G. W. P., Lof, A., Muscarella, L. A., Ehrler, B., Garnett, E. C., & Ginger, D. S. (2019) · Joule · doi:10.1016/j.joule.2019.09.001 · Cited by 273
Recent progress in morphology optimization in perovskite solar cell
Tailor, N. K., Abdi-Jalebi, M., Gupta, V., Hu, H., Dar, M. I., Li, G., & Satapathi, S. (2020) · Journal of Materials Chemistry A · doi:10.1039/d0ta00143k · Cited by 268
Metadata
- Authors
- Dou, B., Whitaker, J. B., Bruening, K., Moore, D. T., Wheeler, L. M., Ryter, J., Breslin, N. J., Berry, J. J., Garner, S. M., Barnes, F. S., Shaheen, S. E., Tassone, C. J., Zhu, K., & van Hest, M. F. A. M.
- Venue
- ACS Energy Letters
- Publisher
- American Chemical Society (ACS)
- Published
- 2018-09-26
- Volume
- 3
- Issue
- 10
- Pages
- 2558-2565
- ISSN
- 2380-8195 (ISSN-L)
- OpenAlex
- W2892717697
- Cited by
- 304
- References
- 36
- FWCI
- 11.01
- Type
- journal article
- Language
- en
- Open access
- closed
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- Dou, B., Whitaker, J. B., Bruening, K., Moore, D. T., Wheeler, L. M., Ryter, J., Breslin, N. J., Berry, J. J., Garner, S. M., Barnes, F. S., Shaheen, S. E., Tassone, C. J., Zhu, K., & van Hest, M. F. A. M. (2018). Roll-to-Roll Printing of Perovskite Solar Cells. ACS Energy Letters. https://doi.org/10.1021/acsenergylett.8b01556
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