The DOI matches its Crossref record; 5 of the 5 references it cites were found in a registry or an index.
Deep Reconstruction of Nickel-Based Precatalysts for Water Oxidation Catalysis
Abstract
Oxygen evolution reaction (OER)-induced reconstruction on precatalysts generally results in surface-reconstructed catalysts with less active species and thus low mass activity. Herein, the deeply reconstructed (DR) catalyst is proposed and derived from a sub-10 nm precatalyst to achieve high-mass-activity catalysis. As a proof-of-concept, the DR-NiOOH with a multilevel nanosheet structure interconnected by sub-5 nm nanoparticles was obtained via a lithiation-induced deep reconstruction strategy. The robust DR-NiOOH with abundant active species enables its significantly enhanced mass activity (170 mV decrease in OER overpotential to achieve 5 mA mg –1 ) and better durability (>10 days) than that of incompletely reconstructed [email protected] Its strong corrosion resistance (30 wt % KOH, 72 h) and high thermal stability (52.8 °C, >40 h) were also confirmed. Theoretical analyses support that the unsaturated OH coverages on orthorhombic NiOOH endow its good OER-active property. This work highlights the merits of high-utilization DR catalysts toward potential catalytic applications under realistic conditions.
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Combining theory and experiment in electrocatalysis: Insights into materials design
Seh, Z. W., Kibsgaard, J., Dickens, C. F., Chorkendorff, I., Nørskov, J. K., & Jaramillo, T. F. (2017) · Science · doi:10.1126/science.aad4998 · Cited by 12,114
Design of electrocatalysts for oxygen- and hydrogen-involving energy conversion reactions
Jiao, Y., Zheng, Y., Jaroniec, M., & Qiao, S. Z. (2015) · Chemical Society Reviews · doi:10.1039/c4cs00470a · Cited by 5,388
Homogeneously dispersed multimetal oxygen-evolving catalysts
Zhang, B., Zheng, X., Voznyy, O., Comin, R., Bajdich, M., García-Melchor, M., Han, L., Xu, J., Liu, M., Zheng, L., et al. (2016) · Science · doi:10.1126/science.aaf1525 · Cited by 2,447
Deng, J., Ren, P., Deng, D., & Bao, X. (2015) · Angewandte Chemie International Edition · doi:10.1002/anie.201409524 · Cited by 1,314
Wang, H., Lee, H.-W., Deng, Y., Lu, Z., Hsu, P.-C., Liu, Y., Lin, D., & Cui, Y. (2015) · Nature Communications · doi:10.1038/ncomms8261 · Cited by 1,257
Cited by
Chen, F.-Y., Wu, Z.-Y., Adler, Z., & Wang, H. (2021) · Joule · doi:10.1016/j.joule.2021.05.005 · Cited by 1,284
Gao, L., Cui, X., Sewell, C. D., Li, J., & Lin, Z. (2021) · Chemical Society Reviews · doi:10.1039/d0cs00962h · Cited by 1,038
Self-supported electrocatalysts for practical water electrolysis
Yang, H., Driess, M., & Menezes, P. W. (2021) · Advanced Energy Materials · doi:10.1002/aenm.202102074 · Cited by 489
Liu, X., Meng, J., Zhu, J., Huang, M., Wen, B., Guo, R., & Mai, L. (2021) · Advanced Materials · doi:10.1002/adma.202007344 · Cited by 438
Self-citationSurface Reconstruction of Water Splitting Electrocatalysts
Zeng, Y., Zhao, M., Huang, Z., Zhu, W., Zheng, J., Jiang, Q., Wang, Z., & Liang, H. (2022) · Advanced Energy Materials · doi:10.1002/aenm.202201713 · Cited by 403
Metadata
- Authors
- Liu, X., Ni, K., Wen, B., Guo, R., Niu, C., Meng, J., Li, Q., Wu, P., Zhu, Y., Wu, X., & Mai, L.
- Venue
- ACS Energy Letters
- Publisher
- American Chemical Society (ACS)
- Published
- 2019-09-27
- Volume
- 4
- Issue
- 11
- Pages
- 2585-2592
- ISSN
- 2380-8195 (ISSN-L)
- OpenAlex
- W2977238283
- Cited by
- 226
- References
- 5
- FWCI
- 4.79
- Type
- journal article
- Language
- en
- Open access
- closed
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- Liu, X., Ni, K., Wen, B., Guo, R., Niu, C., Meng, J., Li, Q., Wu, P., Zhu, Y., Wu, X., & Mai, L. (2019). Deep Reconstruction of Nickel-Based Precatalysts for Water Oxidation Catalysis. ACS Energy Letters. https://doi.org/10.1021/acsenergylett.9b01922
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