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Simple Benchtop Approach to Polymer Brush Nanostructures Using Visible-Light-Mediated Metal-Free Atom Transfer Radical Polymerization
Open accessAbstract
The development of an operationally simple, metal-free surface-initiated atom transfer radical polymerization (SI-ATRP) based on visible-light mediation is reported. The facile nature of this process enables the fabrication of well-defined polymer brushes from flat and curved surfaces using a "benchtop" setup that can be easily scaled to four-inch wafers. This circumvents the requirement of stringent air-free environments (i.e., glovebox), and mediation by visible light allows for spatial control on the micron scale, with complex three-dimensional patterns achieved in a single step. This robust approach leads to unprecedented access to brush architectures for nonexperts.
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Barbey, R., Lavanant, L., Paripovic, D., Schüwer, N., Sugnaux, C., Tugulu, S., & Klok, H.-A. (2009) · Chemical Reviews · doi:10.1021/cr900045a · Cited by 1,753
Cited by
Pearson, R. M., Lim, C.-H., McCarthy, B. G., Musgrave, C. B., & Miyake, G. M. (2016) · Journal of the American Chemical Society · doi:10.1021/jacs.6b08068 · Cited by 339
Wu, C., Corrigan, N., Lim, C.-H., Liu, W., Miyake, G., & Boyer, C. (2022) · Chemical Reviews · doi:10.1021/acs.chemrev.1c00409 · Cited by 259
Wang, P., Dai, J., Ma, Y., Chen, L., & Pan, J. (2020) · Chemical Engineering Journal · doi:10.1016/j.cej.2019.122495 · Cited by 59
Metadata
- Authors
- Discekici, E. H., Pester, C. W., Treat, N. J., Lawrence, J., Mattson, K. M., Narupai, B., Toumayan, E. P., Luo, Y., McGrath, A. J., Clark, P. G., Read de Alaniz, J., & Hawker, C. J.
- Venue
- ACS Macro Letters
- Publisher
- American Chemical Society (ACS)
- Published
- 2016-02-02
- Volume
- 5
- Issue
- 2
- Pages
- 258-262
- ISSN
- 2161-1653 (ISSN-L)
- OpenAlex
- W2265516849
- Cited by
- 203
- References
- 1
- FWCI
- 16.78
- Type
- journal article
- Language
- en
- Open access
- green
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- The paper
- Discekici, E. H., Pester, C. W., Treat, N. J., Lawrence, J., Mattson, K. M., Narupai, B., Toumayan, E. P., Luo, Y., McGrath, A. J., Clark, P. G., Read de Alaniz, J., & Hawker, C. J. (2016). Simple Benchtop Approach to Polymer Brush Nanostructures Using Visible-Light-Mediated Metal-Free Atom Transfer Radical Polymerization. ACS Macro Letters. https://doi.org/10.1021/acsmacrolett.6b00004
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
