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Surface Modified Nanocellulose Fibers Yield Conducting Polymer-Based Flexible Supercapacitors with Enhanced Capacitances
Abstract
We demonstrate that surface modified nanocellulose fibers (NCFs) can be used as substrates to synthesize supercapacitor electrodes with the highest full electrode-normalized gravimetric (127 F g(-1)) and volumetric (122 F cm(-3)) capacitances at high current densities (300 mA cm(-2) ≈ 33 A g(-1)) until date reported for conducting polymer-based electrodes with active mass loadings as high as 9 mg cm(-2). By introducing quaternary amine groups on the surface of NCFs prior to polypyrrole (PPy) polymerization, the macropore volume of the formed PPy-NCF composites can be minimized while maintaining the volume of the micro- and mesopores at the same level as when unmodified or carboxylate groups functionalized NCFs are employed as polymerization substrates. Symmetric, aqueous electrolyte-based, devices comprising these porosity-optimized electrodes exhibit device-specific volumetric energy and power densities of 3.1 mWh cm(-3) and 3 W cm(-3) respectively; which are among the highest values reported for conducting polymer electrodes in aqueous electrolytes. The functionality of the devices is verified by powering a red light-emitting diode with the device in different mechanically challenging states.
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Metadata
- Authors
- Wang, Z., Carlsson, D. O., Tammela, P., Hua, K., Zhang, P., Nyholm, L., & Strømme, M.
- Venue
- ACS Nano
- Publisher
- American Chemical Society (ACS)
- Published
- 2015-06-22
- Volume
- 9
- Issue
- 7
- Pages
- 7563-7571
- ISSN
- 1936-0851 (ISSN-L)
- 1936-086X
- OpenAlex
- W1786317728
- Cited by
- 273
- References
- 37
- FWCI
- 9.76
- Type
- journal article
- Language
- en
- Open access
- closed
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