The DOI matches its Crossref record; 3 of the 3 references it cites were found in a registry or an index.
Atomically Thin Mesoporous Nanomesh of Graphitic C3N4 for High-Efficiency Photocatalytic Hydrogen Evolution
Abstract
Delamination of layer materials into two-dimensional single-atom sheets has induced exceptional physical properties, including large surface area, ultrahigh intrinsic carrier mobility, pronounced changes in the energy band structure, and other properties. Here, atomically thin mesoporous nanomesh of graphitic carbon nitride (g-C3N4) is fabricated by solvothermal exfoliation of mesoporous g-C3N4 bulk made from thermal polymerization of freeze-drying assembled Dicyandiamide nanostructure precursor. With the unique structural advantages for aligned energy levels, electron transfer, light harvesting, and the richly available reaction sites, the as-prepared monolayer of mesoporous g-C3N4 nanomesh exhibits a superior photocatalytic hydrogen evolution rate of 8510 μmol h(-1) g(-1) under λ > 420 nm and an apparent quantum efficiency of 5.1% at 420 nm, the highest of all the metal-free g-C3N4 nanosheets photocatalysts.
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Citations
Cites
Electric Field Effect in Atomically Thin Carbon Films
Novoselov, K. S., Geim, A. K., Morozov, S. V., Jiang, D., Zhang, Y., Dubonos, S. V., Grigorieva, I. V., & Firsov, A. A. (2004) · Science · doi:10.1126/science.1102896 · Cited by 66,834
Geim, A. K., & Novoselov, K. S. (2007) · Nature Materials · doi:10.1038/nmat1849 · Cited by 39,979
A Graphitic‐C 3 N 4 “Seaweed” Architecture for Enhanced Hydrogen Evolution
Han, Q., Wang, B., Zhao, Y., Hu, C., & Qu, L. (2015) · Angewandte Chemie International Edition · doi:10.1002/anie.201504985 · Cited by 472
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Cited by
Ong, W.-J., Tan, L.-L., Ng, Y. H., Yong, S.-T., & Chai, S.-P. (2016) · Chemical Reviews · doi:10.1021/acs.chemrev.6b00075 · Cited by 7,147
Selective Breaking of Hydrogen Bonds of Layered Carbon Nitride for Visible Light Photocatalysis
Kang, Y., Yang, Y., Yin, L., Kang, X., Wang, L., Liu, G., & Cheng, H. (2016) · Advanced Materials · doi:10.1002/adma.201601567 · Cited by 626
Zeng, M., Xiao, Y., Liu, J., Yang, K., & Fu, L. (2018) · Chemical Reviews · doi:10.1021/acs.chemrev.7b00633 · Cited by 574
Ren, Y., Zeng, D., & Ong, W.-J. (2019) · Chinese Journal of Catalysis · doi:10.1016/s1872-2067(19)63293-6 · Cited by 528
Li, B., Lai, C., Zeng, G., Huang, D., Qin, L., Zhang, M., Cheng, M., Liu, X., Yi, H., Zhou, C., et al. (2019) · Small · doi:10.1002/smll.201804565 · Cited by 367
Metadata
- Authors
- Han, Q., Wang, B., Gao, J., Cheng, Z., Zhao, Y., Zhang, Z., & Qu, L.
- Venue
- ACS Nano
- Publisher
- American Chemical Society (ACS)
- Published
- 2016-01-21
- Volume
- 10
- Issue
- 2
- Pages
- 2745-2751
- ISSN
- 1936-0851 (ISSN-L)
- 1936-086X
- OpenAlex
- W2239593222
- Cited by
- 978
- References
- 3
- FWCI
- 39.60
- Type
- journal article
- Language
- en
- Open access
- closed
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- Han, Q., Wang, B., Gao, J., Cheng, Z., Zhao, Y., Zhang, Z., & Qu, L. (2016). Atomically Thin Mesoporous Nanomesh of Graphitic C3N4 for High-Efficiency Photocatalytic Hydrogen Evolution. ACS Nano. https://doi.org/10.1021/acsnano.5b07831
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