The DOI matches its Crossref record; 2 of the 2 references it cites were found in a registry or an index.
Quantum Mechanical Description of Raman Scattering from Molecules in Plasmonic Cavities
Open accessAbstract
Plasmon-enhanced Raman scattering can push single-molecule vibrational spectroscopy beyond a regime addressable by classical electrodynamics. We employ a quantum electrodynamics (QED) description of the coherent interaction of plasmons and molecular vibrations that reveal the emergence of nonlinearities in the inelastic response of the system. For realistic situations, we predict the onset of phonon-stimulated Raman scattering and a counterintuitive dependence of the anti-Stokes emission on the frequency of excitation. We further show that this QED framework opens a venue to analyze the correlations of photons emitted from a plasmonic cavity.
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Citations
Cites
On the generators of quantum dynamical semigroups
Lindblad, G. (1976) · Communications in Mathematical Physics · doi:10.1007/bf01608499 · Cited by 7,548
Completely positive dynamical semigroups of N -level systems
Gorini, V., Kossakowski, A., & Sudarshan, E. C. G. (1976) · Journal of Mathematical Physics · doi:10.1063/1.522979 · Cited by 3,998
Metadata
- Authors
- Schmidt, M. K., Esteban, R., González-Tudela, A., Giedke, G., & Aizpurua, J.
- Venue
- ACS Nano
- Publisher
- American Chemical Society (ACS)
- Published
- 2016-05-31
- Volume
- 10
- Issue
- 6
- Pages
- 6291-6298
- ISSN
- 1936-0851 (ISSN-L)
- 1936-086X
- OpenAlex
- W1850806008
- Cited by
- 179
- References
- 2
- FWCI
- 9.58
- Type
- journal article
- Language
- en
- Open access
- green
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- Schmidt, M. K., Esteban, R., González-Tudela, A., Giedke, G., & Aizpurua, J. (2016). Quantum Mechanical Description of Raman Scattering from Molecules in Plasmonic Cavities. ACS Nano. https://doi.org/10.1021/acsnano.6b02484
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