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Ultrafast Nonlinear Excitation Dynamics of Black Phosphorus Nanosheets from Visible to Mid-Infrared

Wang, Kangpeng, Szydłowska, Beata M., Wang, Gaozhong, Zhang, Xiaoyan, Wang, Jing Jing, Magan, John J., Zhang, Long, Coleman, Jonathan N., Wang, Jun, Blau, Werner J.·2016·ACS Nano

Abstract

The recent progress on black phosphorus makes it a promising candidate material for broadband nanophotonic devices, especially operating in the mid-infrared spectral region. Here, the excited carrier dynamics and nonlinear optical response of unoxidized black phosphorus nanosheets and their wavelength dependence were systematically studied from 800 nm to 2.1 μm. The wavelength-dependent relaxation times of black phosphorus nanosheets are determined to be 360 fs to 1.36 ps with photon energies from 1.55 to 0.61 eV. In a comparative study with graphene, we found that black phosphorus has a faster carrier relaxation in near- and mid-infrared region. With regard to nonlinear optical absorption, the response of black phosphorus significantly increases from near- to mid-infrared, and black phosphorus is also confirmed to be better as saturable absorber to MoS2 in infrared region.

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Metadata

Authors
Wang, K., Szydłowska, B. M., Wang, G., Zhang, X., Wang, J. J., Magan, J. J., Zhang, L., Coleman, J. N., Wang, J., & Blau, W. J.
Venue
ACS Nano
Published
2016-06-16
Volume
10
Issue
7
Pages
6923-6932
ISSN
  • 1936-0851 (ISSN-L)
  • 1936-086X
OpenAlex
W2419241806
Cited by
295
References
0
FWCI
13.10
Type
journal article
Language
en
Open access
closed

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CoChat. (2026). Citation check: Ultrafast Nonlinear Excitation Dynamics of Black Phosphorus Nanosheets from Visible to Mid-Infrared. https://app.cochat.ai/papers/10.1021/acsnano.6b02770
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Wang, K., Szydłowska, B. M., Wang, G., Zhang, X., Wang, J. J., Magan, J. J., Zhang, L., Coleman, J. N., Wang, J., & Blau, W. J. (2016). Ultrafast Nonlinear Excitation Dynamics of Black Phosphorus Nanosheets from Visible to Mid-Infrared. ACS Nano. https://doi.org/10.1021/acsnano.6b02770

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