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Laser Crystallization of Organic–Inorganic Hybrid Perovskite Solar Cells
Abstract
Organic-inorganic hybrid perovskites attract enormous research interest for next generation solar energy harvest. Synergistic crystalline structures comprising organic and inorganic components enable solution processing of perovskite films. A reliable crystallization method for perovskites, compatible with fast continuous process over large-area flexible substrates, is crucial for high performance solar cell production. Here, we present laser crystallization of hybrid perovskite solar cells using near-infrared (NIR) laser (λ = 1064 nm). Crystalline morphology of CH3NH3PbI3 (MAPbI3) perovskite films are widely controllable with laser irradiation condition while maintaining film uniformity. Photothermal heating effectively assisted by interfacial photoconversion layers is critical for phase transformation without beam damage of multilayered device structures. Notably, laser crystallization attains higher device performances than conventional thermal annealing. Fast laser crystallization with manufacture level scan rate (1 m min(-1)) demonstrates inverted-type perovskite solar cells with 11.3 and 8.0% efficiencies on typical glass and flexible polymer substrates, respectively, without rigorous device optimization.
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Cites
Solvent engineering for high-performance inorganic–organic hybrid perovskite solar cells
Jeon, N. J., Noh, J. H., Kim, Y. C., Yang, W. S., Ryu, S., & Seok, S. I. (2014) · Nature Materials · doi:10.1038/nmat4014 · Cited by 6,723
Optical Properties of Condensed Matter and Applications
(2006) · doi:10.1002/0470021942 · Cited by 294
Cited by
Synthetic Approaches for Halide Perovskite Thin Films
Dunlap-Shohl, W. A., Zhou, Y., Padture, N. P., & Mitzi, D. B. (2019) · Chemical Reviews · doi:10.1021/acs.chemrev.8b00318 · Cited by 631
Kim, Y.-H., Wolf, C., Kim, Y.-T., Cho, H., Kwon, W., Do, S., Sadhanala, A., Park, C. G., Rhee, S.-W., Im, S. H., et al. (2017) · ACS Nano · doi:10.1021/acsnano.6b07617 · Cited by 375
Al Zoubi, W., Kamil, M. P., Fatimah, S., Nashrah, N., & Ko, Y. G. (2020) · Progress in Materials Science · doi:10.1016/j.pmatsci.2020.100663 · Cited by 265
Direct laser writing on halide perovskites: from mechanisms to applications
Sheng, Y., Wen, X., Jia, B., & Gan, Z. (2024) · Light: Advanced Manufacturing · doi:10.37188/lam.2024.004 · Cited by 22
Metadata
- Authors
- Jeon, T., Jin, H. M., Lee, S. H., Lee, J. M., Park, H. I., Kim, M. K., Lee, K. J., Shin, B., & Kim, S. O.
- Venue
- ACS Nano
- Publisher
- American Chemical Society (ACS)
- Published
- 2016-07-19
- Volume
- 10
- Issue
- 8
- Pages
- 7907-7914
- ISSN
- 1936-0851 (ISSN-L)
- 1936-086X
- OpenAlex
- W2463111809
- Cited by
- 160
- References
- 2
- FWCI
- 8.08
- Type
- journal article
- Language
- en
- Open access
- closed
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- Jeon, T., Jin, H. M., Lee, S. H., Lee, J. M., Park, H. I., Kim, M. K., Lee, K. J., Shin, B., & Kim, S. O. (2016). Laser Crystallization of Organic–Inorganic Hybrid Perovskite Solar Cells. ACS Nano. https://doi.org/10.1021/acsnano.6b03815
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