The DOI matches its Crossref record; 3 of the 3 references it cites were found in a registry or an index.
Multimodality of Structural, Electrical, and Gravimetric Responses of Intercalated MXenes to Water
Abstract
Understanding of structural, electrical, and gravimetric peculiarities of water vapor interaction with ion-intercalated MXenes led to design of a multimodal humidity sensor. Neutron scattering coupled to molecular dynamics and ab initio calculations showed that a small amount of hydration results in a significant increase in the spacing between MXene layers in the presence of K and Mg intercalants between the layers. Films of K- and Mg-intercalated MXenes exhibited relative humidity (RH) detection thresholds of ∼0.8% RH and showed monotonic RH response in the 0–85% RH range. We found that MXene gravimetric response to water is 10 times faster than their electrical response, suggesting that H 2 O-induced swelling/contraction of channels between MXene sheets results in trapping of H 2 O molecules that act as charge-depleting dopants. The results demonstrate the use of MXenes as humidity sensors and infer potential impact of water on structural and electrical performance of MXene-based devices.
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Shannon, R. D. (1976) · Acta Crystallographica Section A · doi:10.1107/s0567739476001551 · Cited by 66,145
Fast Parallel Algorithms for Short-Range Molecular Dynamics
Plimpton, S. (1995) · Journal of Computational Physics · doi:10.1006/jcph.1995.1039 · Cited by 44,721
Phenomenological Theory of Ion Solvation. Effective Radii of Hydrated Ions
Nightingale, E. R. (1959) · The Journal of Physical Chemistry · doi:10.1021/j150579a011 · Cited by 3,505
Cited by
Ten Years of Progress in the Synthesis and Development of MXenes
Naguib, M., Barsoum, M. W., & Gogotsi, Y. (2021) · Advanced Materials · doi:10.1002/adma.202103393 · Cited by 1,257
Self-citationJiang, X., Kuklin, A. V., Baev, A., Ge, Y., Ågren, H., Zhang, H., & Prasad, P. N. (2020) · Physics Reports · doi:10.1016/j.physrep.2019.12.006 · Cited by 914
Effective ion sieving with Ti3C2Tx MXene membranes for production of drinking water from seawater
Ding, L., Li, L., Liu, Y., Wu, Y., Lu, Z., Deng, J., Wei, Y., Caro, J., & Wang, H. (2020) · Nature Sustainability · doi:10.1038/s41893-020-0474-0 · Cited by 804
Self-citationLiu, L., Chen, W., Zhang, H., Wang, Q., Guan, F., & Yu, Z. (2019) · Advanced Functional Materials · doi:10.1002/adfm.201905197 · Cited by 699
Environment-Sensitive Photoresponse of Spontaneously Partially Oxidized Ti3C2 MXene Thin Films
Chertopalov, S., & Mochalin, V. N. (2018) · ACS Nano · doi:10.1021/acsnano.8b02379 · Cited by 308
Metadata
- Authors
- Muckley, E. S., Naguib, M., Wang, H.-W., Vlcek, L., Osti, N. C., Sacci, R. L., Sang, X., Unocic, R. R., Xie, Y., Tyagi, M., Mamontov, E., Page, K. L., Kent, P. R. C., Nanda, J., & Ivanov, I. N.
- Venue
- ACS Nano
- Publisher
- American Chemical Society (ACS)
- Published
- 2017-10-17
- Volume
- 11
- Issue
- 11
- Pages
- 11118-11126
- ISSN
- 1936-0851 (ISSN-L)
- 1936-086X
- OpenAlex
- W2762833022
- Cited by
- 271
- References
- 3
- FWCI
- 7.45
- Type
- journal article
- Language
- en
- Open access
- closed
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- Muckley, E. S., Naguib, M., Wang, H.-W., Vlcek, L., Osti, N. C., Sacci, R. L., Sang, X., Unocic, R. R., Xie, Y., Tyagi, M., Mamontov, E., Page, K. L., Kent, P. R. C., Nanda, J., & Ivanov, I. N. (2017). Multimodality of Structural, Electrical, and Gravimetric Responses of Intercalated MXenes to Water. ACS Nano. https://doi.org/10.1021/acsnano.7b05264
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