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Synthesis of PdM (M = Zn, Cd, ZnCd) Nanosheets with an Unconventional Face-Centered Tetragonal Phase as Highly Efficient Electrocatalysts for Ethanol Oxidation
Abstract
Abstract Recently, crystal-phase engineering has been emerging as a promising strategy to tune the physicochemical properties of noble metal catalysts and further improve their catalytic performance. However, the synthesis of noble metal catalysts with an unconventional crystal phase as well as desired composition and morphology still remains a great challenge. Herein, a series of PdM (M = Zn, Cd, ZnCd) nanosheets (NSs) with thickness less than 5 nm have been synthesized via a facile one-pot wet-chemical method. In particular, different from the conventional face-centered cubic (fcc) phase, PdM NSs possess an unconventional face-centered tetragonal (fct) phase. As a proof-of-concept application, the fct PdZn NSs exhibit significantly enhanced mass activity and stability in ethanol oxidation reaction, compared to the pure Pd NSs and commercial Pd black catalyst.
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Monodisperse FePt Nanoparticles and Ferromagnetic FePt Nanocrystal Superlattices
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Enhanced electrocatalytic CO2 reduction via field-induced reagent concentration
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Freestanding palladium nanosheets with plasmonic and catalytic properties
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New Approach to Fully Ordered fct-FePt Nanoparticles for Much Enhanced Electrocatalysis in Acid
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Cited by
Defect‐Rich Porous Palladium Metallene for Enhanced Alkaline Oxygen Reduction Electrocatalysis
Yu, H., Zhou, T., Wang, Z., Xu, Y., Li, X., Wang, L., & Wang, H. (2021) · Angewandte Chemie International Edition · doi:10.1002/anie.202101019 · Cited by 298
Universal strategies to multi-dimensional noble-metal-based catalysts for electrocatalysis
Gao, F., Zhang, Y., Wu, Z., You, H., & Du, Y. (2021) · Coordination Chemistry Reviews · doi:10.1016/j.ccr.2021.213825 · Cited by 221
Xie, M., Zhang, B., Jin, Z., Li, P., & Yu, G. (2022) · ACS Nano · doi:10.1021/acsnano.2c05190 · Cited by 167
Metadata
- Authors
- Yun, Q., Lu, Q., Li, C., Chen, B., Zhang, Q., He, Q., Hu, Z., Zhang, Z., Ge, Y., Yang, N., Ge, J., He, Y.-B., Gu, L., & Zhang, H.
- Venue
- ACS Nano
- Publisher
- American Chemical Society (ACS)
- Published
- 2019-11-27
- Volume
- 13
- Issue
- 12
- Pages
- 14329-14336
- ISSN
- 1936-0851 (ISSN-L)
- 1936-086X
- OpenAlex
- W2991558899
- Cited by
- 180
- References
- 5
- FWCI
- 4.38
- Type
- journal article
- Language
- en
- Open access
- closed
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- Yun, Q., Lu, Q., Li, C., Chen, B., Zhang, Q., He, Q., Hu, Z., Zhang, Z., Ge, Y., Yang, N., Ge, J., He, Y.-B., Gu, L., & Zhang, H. (2019). Synthesis of PdM (M = Zn, Cd, ZnCd) Nanosheets with an Unconventional Face-Centered Tetragonal Phase as Highly Efficient Electrocatalysts for Ethanol Oxidation. ACS Nano. https://doi.org/10.1021/acsnano.9b07775
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