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High-Thermal-Stability and High-Thermal-Conductivity Ti3C2Tx MXene/Poly(vinyl alcohol) (PVA) Composites
Open accessAbstract
Abstract MXenes, a new family of two-dimensional materials, have recently attracted increasing attention due to their unique properties for a wide range of potential applications. Herein, we synthesize Ti3C2Tx/poly(vinyl alcohol) (PVA) composites and investigate the effects of the thermal properties of MXene by temperature-dependent Raman spectroscopy and polarized-laser power-dependent Raman spectroscopy. Compared to the Ti3C2Tx MXene, the PVA significantly improves the thermal stability of Ti3C2Tx by reducing the thermal coefficient of the Eg1 mode from −0.06271 to −0.03357 cm–1/K, which is attributed to the strong Ti–O bonds formed between the MXene and PVA polymer confirmed by the X-ray photoelectron spectroscopy results. Meanwhile, the thermal conductivities of Ti3C2Tx and Ti3C2Tx/PVA composites reach as high as about 55.8 and 47.6 W/(m K), respectively. Overall, this work will contribute to extend the MXene applications in terms of polymer-based nanocomposites and improve the reliability of the related devices effectively.
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Cites
Superior Thermal Conductivity of Single-Layer Graphene
Balandin, A. A., Ghosh, S., Bao, W., Calizo, I., Teweldebrhan, D., Miao, F., & Lau, C. N. (2008) · Nano Letters · doi:10.1021/nl0731872 · Cited by 13,823
Cited by
Jiang, X., Kuklin, A. V., Baev, A., Ge, Y., Ågren, H., Zhang, H., & Prasad, P. N. (2020) · Physics Reports · doi:10.1016/j.physrep.2019.12.006 · Cited by 914
Antioxidants Unlock Shelf-Stable Ti3C2T (MXene) Nanosheet Dispersions
Zhao, X., Vashisth, A., Prehn, E., Sun, W., Shah, S. A., Habib, T., Chen, Y., Tan, Z., Lutkenhaus, J. L., Radovic, M., et al. (2019) · Matter · doi:10.1016/j.matt.2019.05.020 · Cited by 747
Leaf-inspired multiresponsive MXene-based actuator for programmable smart devices
Cai, G., Ciou, J.-H., Liu, Y., Jiang, Y., & Lee, P. S. (2019) · Science Advances · doi:10.1126/sciadv.aaw7956 · Cited by 341
Mechanotribological Aspects of MXene‐Reinforced Nanocomposites
Malaki, M., & Varma, R. S. (2020) · Advanced Materials · doi:10.1002/adma.202003154 · Cited by 292
MXene aerogel-based phase change materials toward solar energy conversion
Lin, P., Xie, J., He, Y., Lu, X., Li, W., Fang, J., Yan, S., Zhang, L., Sheng, X., & Chen, Y. (2020) · Solar Energy Materials and Solar Cells · doi:10.1016/j.solmat.2019.110229 · Cited by 268
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Metadata
- Authors
- Liu, R., & Li, W.
- Venue
- ACS Omega
- Publisher
- American Chemical Society (ACS)
- Published
- 2018-03-05
- Volume
- 3
- Issue
- 3
- Pages
- 2609-2617
- ISSN
- 2470-1343 (ISSN-L)
- OpenAlex
- W2790959738
- Cited by
- 487
- References
- 1
- FWCI
- 10.66
- Type
- journal article
- Language
- en
- Open access
- gold
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- Liu, R., & Li, W. (2018). High-Thermal-Stability and High-Thermal-Conductivity Ti3C2Tx MXene/Poly(vinyl alcohol) (PVA) Composites. ACS Omega. https://doi.org/10.1021/acsomega.7b02001
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