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Strong Exciton–Photon Coupling and Lasing Behavior in All-Inorganic CsPbBr3 Micro/Nanowire Fabry-Pérot Cavity

Du, Wenna, Zhang, Shuai, Shi, Jia, Chen, Jie, Wu, Zhiyong, Mi, Yang, Liu, Zhixiong, Li, Yuanzheng, Sui, Xinyu, Wang, Rui, Qiu, Xiaohui, Wu, Tom, Xiao, Yunfeng, Zhang, Qing, Liu, Xinfeng·2018·ACS Photonics

Abstract

All-inorganic perovskite micro/nanowire materials hold great promises as nanoscale coherent light source due to their superior optical and electronic properties. The coupling strength between exciton and photon in this system is important for their optical application, however, is rarely studied. In this work, we demonstrated the strong coupling of exciton-photon and polariton lasing in high quality CsPbBr 3 micro/nanowires synthesized by a CVD method. By exploring spatial resolved PL spectra of CsPbBr 3 cavity, we observed mode volume dependent coupling strength with a vacuum Rabi splitting up to 656 meV, as well as significant increase in group index. Moreover, low threshold polariton lasing was achieved at room temperature within strong coupling regime; the polariton characteristic is confirmed by comparing lasing spectra with waveguided output spectra and the dramatically reduced lasing threshold. Our present results provide new avenues to achieve high coupling strengths potentially enabling application of exciting phenomena such as Bose–Einstein condensation of polaritons, efficient light-emitting diodes, and lasers.

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Metadata

Authors
Du, W., Zhang, S., Shi, J., Chen, J., Wu, Z., Mi, Y., Liu, Z., Li, Y., Sui, X., Wang, R., Qiu, X., Wu, T., Xiao, Y., Zhang, Q., & Liu, X.
Venue
ACS Photonics
Published
2018-03-13
Volume
5
Issue
5
Pages
2051-2059
ISSN
2330-4022 (ISSN-L)
OpenAlex
W2963336898
Cited by
180
References
3
FWCI
12.50
Type
journal article
Language
en
Open access
closed

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CoChat. (2026). Citation check: Strong Exciton–Photon Coupling and Lasing Behavior in All-Inorganic CsPbBr3 Micro/Nanowire Fabry-Pérot Cavity. https://app.cochat.ai/papers/10.1021/acsphotonics.7b01593
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Du, W., Zhang, S., Shi, J., Chen, J., Wu, Z., Mi, Y., Liu, Z., Li, Y., Sui, X., Wang, R., Qiu, X., Wu, T., Xiao, Y., Zhang, Q., & Liu, X. (2018). Strong Exciton–Photon Coupling and Lasing Behavior in All-Inorganic CsPbBr3 Micro/Nanowire Fabry-Pérot Cavity. ACS Photonics. https://doi.org/10.1021/acsphotonics.7b01593

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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).

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