The DOI matches its Crossref record; 2 of the 2 references it cites were found in a registry or an index.
One-Pot Catalytic Conversion of Raw Lignocellulosic Biomass into Gasoline Alkanes and Chemicals over LiTaMoO6 and Ru/C in Aqueous Phosphoric Acid
Abstract
Lignocellulosic biomass is a renewable feedstock that has the potential to replace the diminishing fossil fuels. Herein, we reported the simultaneous conversion of cellulose, hemicellulose and lignin from raw biomass into gasoline alkanes (hexanes and pentanes) and monophenols and related hydrocarbons over layered LiTaMoO 6 and Ru/C in aqueous phosphoric acid medium. Specifically, gasoline alkanes were directly yielded from the carbohydrate components, based on hemicellulose and cellulose, and the total yield could be up to 82.4%. Notably, the lignin fraction could also be transformed into monophenols, related alcohols and hydrocarbons by the one-pot reaction. It suggested that the hydrocracking of monophenol fraction could be performed in this catalytic system. The total yield of volatile products was 53% based on the lignin fraction. In this paper, the influences of phosphoric acid concentration, substrate ash and the amino acids derived from the biogenic impurities were investigated and different raw biomass substrates were tested. Furthermore, the catalysts could be reused for several runs to convert raw biomass without pretreatment.
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Cites
The Catalytic Valorization of Lignin for the Production of Renewable Chemicals
Zakzeski, J., Bruijnincx, P. C. A., Jongerius, A. L., & Weckhuysen, B. M. (2010) · Chemical Reviews · doi:10.1021/cr900354u · Cited by 4,468
Lignin depolymerisation strategies: towards valuable chemicals and fuels
Xu, C., Arancon, R. A. D., Labidi, J., & Luque, R. (2014) · Chem. Soc. Rev. · doi:10.1039/c4cs00235k · Cited by 1,031
Cited by
Catalytic conversion of lignocellulosic biomass into chemicals and fuels
Deng, W., Feng, Y., Fu, J., Guo, H., Guo, Y., Han, B., Jiang, Z., Kong, L., Li, C., Liu, H., et al. (2023) · Green Energy & Environment · doi:10.1016/j.gee.2022.07.003 · Cited by 854
Lignin-first biomass fractionation: the advent of active stabilisation strategies
Renders, T., Van den Bosch, S., Koelewijn, S.-F., Schutyser, W., & Sels, B. F. (2017) · Energy & Environmental Science · doi:10.1039/c7ee01298e · Cited by 709
Galkin, M. V., & Samec, J. S. M. (2016) · ChemSusChem · doi:10.1002/cssc.201600237 · Cited by 640
Tomishige, K., Nakagawa, Y., & Tamura, M. (2017) · Green Chemistry · doi:10.1039/c7gc00620a · Cited by 284
Biofuels and renewable chemicals production by catalytic pyrolysis of cellulose: a review
Hassan, N. S., Jalil, A. A., Hitam, C. N. C., Vo, D. V. N., & Nabgan, W. (2020) · Environmental Chemistry Letters · doi:10.1007/s10311-020-01040-7 · Cited by 176
Metadata
- Authors
- Liu, Y., Chen, L., Wang, T., Zhang, Q., Wang, C., Yan, J., & Ma, L.
- Venue
- ACS Sustainable Chemistry & Engineering
- Publisher
- American Chemical Society (ACS)
- Published
- 2015-07-07
- Volume
- 3
- Issue
- 8
- Pages
- 1745-1755
- ISSN
- 2168-0485 (ISSN-L)
- OpenAlex
- W1658735240
- Cited by
- 184
- References
- 2
- FWCI
- 9.91
- Type
- journal article
- Language
- en
- Open access
- closed
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- Liu, Y., Chen, L., Wang, T., Zhang, Q., Wang, C., Yan, J., & Ma, L. (2015). One-Pot Catalytic Conversion of Raw Lignocellulosic Biomass into Gasoline Alkanes and Chemicals over LiTaMoO6 and Ru/C in Aqueous Phosphoric Acid. ACS Sustainable Chemistry & Engineering. https://doi.org/10.1021/acssuschemeng.5b00256
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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