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Photoreactivity and Mechanism of g-C3N4 and Ag Co-Modified Bi2WO6 Microsphere under Visible Light Irradiation
Abstract
In this study, C 3 N 4 @Ag-Bi 2 WO 6 with flower-like architecture was successfully prepared through a facile process. The C 3 N 4 @Ag-Bi 2 WO 6 particles with 2–4 μm diameters present remarkable enhanced visible light absorption and electron–hole separation efficiency. Compared with Bi 2 WO 6, Ag-Bi 2 WO 6, and C 3 N 4 @Bi 2 WO 6 systems, the C 3 N 4 @Ag-Bi 2 WO 6 system exhibits optimal photocatalytic activities in both the degradation of RhB and hydrogen production out of water under visible light irradiation. We propose that these results are attributed to the synergy effects of Ag, g-C 3 N 4, and Bi 2 WO 6 nanophase structures in the C 3 N 4 @Ag-Bi 2 WO 6 composites, which results in a fast electron–hole separation and slow charge recombination by a Z-scheme mechanism and ultimately in a higher photocatalytic activity.
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Cites
Metal-free efficient photocatalyst for stable visible water splitting via a two-electron pathway
Liu, J., Liu, Y., Liu, N., Han, Y., Zhang, X., Huang, H., Lifshitz, Y., Lee, S.-T., Zhong, J., & Kang, Z. (2015) · Science · doi:10.1126/science.aaa3145 · Cited by 4,468
Catalytic nanoarchitectures—The importance of nothing and the unimportance of periodicity
Rolison, D. R. (2003) · Science · doi:10.1126/science.1082332 · Cited by 1,037
Cited by
Xia, P., Zhu, B., Cheng, B., Yu, J., & Xu, J. (2018) · ACS Sustainable Chemistry & Engineering · doi:10.1021/acssuschemeng.7b03289 · Cited by 630
Chen, F., Yang, Q., Wang, Y., Zhao, J., Wang, D., Li, X., Guo, Z., Wang, H., Deng, Y., Niu, C., et al. (2017) · Applied Catalysis B: Environmental · doi:10.1016/j.apcatb.2016.12.017 · Cited by 429
Recent development in graphitic carbon nitride based photocatalysis for hydrogen generation
Nasir, M. S., Yang, G., Ayub, I., Wang, S., Wang, L., Wang, X., Yan, W., Peng, S., & Ramakarishna, S. (2019) · Applied Catalysis B: Environmental · doi:10.1016/j.apcatb.2019.117855 · Cited by 351
Jo, W.-K., Kumar, S., Eslava, S., & Tonda, S. (2018) · Applied Catalysis B: Environmental · doi:10.1016/j.apcatb.2018.08.056 · Cited by 344
Teixeira, I. F., Barbosa, E. C. M., Tsang, S. C. E., & Camargo, P. H. C. (2018) · Chemical Society Reviews · doi:10.1039/c8cs00479j · Cited by 316
Metadata
- Authors
- Xiao, X., Wei, J., Yang, Y., Xiong, R., Pan, C., & Shi, J.
- Venue
- ACS Sustainable Chemistry & Engineering
- Publisher
- American Chemical Society (ACS)
- Published
- 2016-05-09
- Volume
- 4
- Issue
- 6
- Pages
- 3017-3023
- ISSN
- 2168-0485 (ISSN-L)
- OpenAlex
- W2342479426
- Cited by
- 178
- References
- 2
- FWCI
- 7.06
- Type
- journal article
- Language
- en
- Open access
- closed
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- CoChat. (2026). Citation check: Photoreactivity and Mechanism of g-C3N4 and Ag Co-Modified Bi2WO6 Microsphere under Visible Light Irradiation. https://app.cochat.ai/papers/10.1021/acssuschemeng.5b01701
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- Xiao, X., Wei, J., Yang, Y., Xiong, R., Pan, C., & Shi, J. (2016). Photoreactivity and Mechanism of g-C3N4 and Ag Co-Modified Bi2WO6 Microsphere under Visible Light Irradiation. ACS Sustainable Chemistry & Engineering. https://doi.org/10.1021/acssuschemeng.5b01701
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