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Highly Efficient Visible-Light-Induced Photoactivity of Z-Scheme g-C3N4/Ag/MoS2 Ternary Photocatalysts for Organic Pollutant Degradation and Production of Hydrogen
Abstract
A Z-scheme g-C 3 N 4 /Ag/MoS 2 ternary plasmonic photocatalyst in a flowerlike architecture of diameter about 0.4–0.6 μm is successfully synthesized by a reliable and effective method. The as-synthesized g-C 3 N 4 /Ag/MoS 2 photocatalyst showed excellent improvement for visible-light absorption and separation efficiency of photoinduced electron–hole pairs. The g-C 3 N 4 /Ag/MoS 2 system exhibits optimum visible-light-induced photocatalytic activity in degrading Rhodamin B (RhB), which is 9.43-fold and 3.56-fold of Ag/MoS 2 and g-C 3 N 4 /MoS 2 systems, and 8.78-fold and 2.08-fold in the production of hydrogen (H 2 ) out of water, respectively. The excellent photocatalytic activities are attributed to the synergetic effects of Ag, g-C 3 N 4, and MoS 2 nanophase structures in the g-C 3 N 4 /Ag/MoS 2 composites, which result in a Z-scheme-mechanism-assisted fast separation and slow recombination of photoinduced electron–hole pairs and thereby higher photocatalytic activity.
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Cites
Chang, K., & Chen, W. (2011) · ACS Nano · doi:10.1021/nn200659w · Cited by 1,663
Catalytic nanoarchitectures—The importance of nothing and the unimportance of periodicity
Rolison, D. R. (2003) · Science · doi:10.1126/science.1082332 · Cited by 1,037
Cited by
Ren, Y., Zeng, D., & Ong, W.-J. (2019) · Chinese Journal of Catalysis · doi:10.1016/s1872-2067(19)63293-6 · Cited by 528
Kumaravel, V., Imam, M., Badreldin, A., Chava, R., Do, J., Kang, M., & Abdel-Wahab, A. (2019) · Catalysts · doi:10.3390/catal9030276 · Cited by 435
Kumar, A., Kumar, A., Sharma, G., Al-Muhtaseb, A. H., Naushad, M., Ghfar, A. A., Guo, C., & Stadler, F. J. (2018) · Chemical Engineering Journal · doi:10.1016/j.cej.2018.01.105 · Cited by 312
Kampouri, S., & Stylianou, K. C. (2019) · ACS Catalysis · doi:10.1021/acscatal.9b00332 · Cited by 298
Metadata
- Authors
- Lu, D., Wang, H., Zhao, X., Kondamareddy, K. K., Ding, J., Li, C., & Fang, P.
- Venue
- ACS Sustainable Chemistry & Engineering
- Publisher
- American Chemical Society (ACS)
- Published
- 2017-01-06
- Volume
- 5
- Issue
- 2
- Pages
- 1436-1445
- ISSN
- 2168-0485 (ISSN-L)
- OpenAlex
- W2563425832
- Cited by
- 395
- References
- 2
- FWCI
- 12.51
- Type
- journal article
- Language
- en
- Open access
- closed
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- Lu, D., Wang, H., Zhao, X., Kondamareddy, K. K., Ding, J., Li, C., & Fang, P. (2017). Highly Efficient Visible-Light-Induced Photoactivity of Z-Scheme g-C3N4/Ag/MoS2 Ternary Photocatalysts for Organic Pollutant Degradation and Production of Hydrogen. ACS Sustainable Chemistry & Engineering. https://doi.org/10.1021/acssuschemeng.6b02010
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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