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One-Step Preparation of Graphene-Supported Anatase TiO2 with Exposed {001} Facets and Mechanism of Enhanced Photocatalytic Properties
Abstract
Anatase TiO2 nanosheets supported on reduced graphene oxide (RGO) were synthesized via a one-step, solvothermal method. During the solvothermal step, graphene oxide (GO) was reduced to RGO, and, subsequently, anatase TiO2 with 73.7% exposed {001} facets was grown in situ on the surfaces of the RGO nanosheets. Compared with pure TiO2, the RGO/TiO2 hybrid nanocomposite had improved photoactivity as a result of effective photoinduced electron transfer from TiO2 to the RGO acceptor through interfacial interactions. Trapping tests showed that the oxidation of dye molecules proceeded for about 22% through the reaction with (•)OH radicals, and the remaining 78% occurred via direct interactions with holes. The holes left in TiO2 crystals were the main reason for the enhanced photocatalytic properties of the RGO/TiO2 composite. This paper not only reports the fabrication of highly active photocatalysts but also gives deeper insight into the photocatalytic mechanism of carbon/TiO2 composites.
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Liu, J., Bai, H., Wang, Y., Liu, Z., Zhang, X., & Sun, D. D. (2010) · Advanced Functional Materials · doi:10.1002/adfm.201001391 · Cited by 776
Cited by
Facet‐Engineered Surface and Interface Design of Photocatalytic Materials
Bai, S., Wang, L., Li, Z., & Xiong, Y. (2017) · Advanced Science · doi:10.1002/advs.201600216 · Cited by 429
Ong, W., Tan, L., Chai, S., Yong, S., & Mohamed, A. R. (2014) · ChemSusChem · doi:10.1002/cssc.201300924 · Cited by 339
Metadata
- Authors
- Gu, L., Wang, J., Cheng, H., Zhao, Y., Liu, L., & Han, X.
- Venue
- ACS Applied Materials & Interfaces
- Publisher
- American Chemical Society (ACS)
- Published
- 2013-04-10
- Volume
- 5
- Issue
- 8
- Pages
- 3085-3093
- ISSN
- 1944-8244 (ISSN-L)
- 1944-8252
- OpenAlex
- W2333226394
- Cited by
- 249
- References
- 1
- FWCI
- 11.78
- Type
- journal article
- Language
- en
- Open access
- closed
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- The paper
- Gu, L., Wang, J., Cheng, H., Zhao, Y., Liu, L., & Han, X. (2013). One-Step Preparation of Graphene-Supported Anatase TiO2 with Exposed {001} Facets and Mechanism of Enhanced Photocatalytic Properties. ACS Applied Materials & Interfaces. https://doi.org/10.1021/am303274t
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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