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Graphene-Wrapped Polyaniline Hollow Spheres As Novel Hybrid Electrode Materials for Supercapacitor Applications
Abstract
Polyaniline hollow spheres (PANI-HS)@electrochemical reduced graphene oxide (ERGO) hybrids with core-shell structures have been fabricated via a solution-based coassembly process. The hollow nanostructured designing for the PANI-HS greatly enlarges the specific surface area, providing high electroactive regions and short diffusion lengths for both charge and ion transport. The wrapping of ERGO sheets on the PANI-HS can offer highly conductive pathways by bridging individual PANI-HS together, thus facilitating the rate and cycling performance of supercapacitors. The specific capacitance of PANI-HS36@ERGO hybrids can reach 614 F g(-1) at a current density of 1 A g(-1). Furthermore, the capacitance of the PANI-HS36@ERGO hybrids maintains 90% after 500 charging/discharging cycles at a current density of 1 A g(-1), indicating a good cycling stability. The greatly enhanced electrochemical performance can be ascribed to the synergic effects of the two components of PANI-HS and ERGO, suggesting that the PANI-HS@ERGO hybrids as novel electrode materials may have potential applications in high-performance energy storage devices.
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Cites
Experimental observation of the quantum Hall effect and Berry's phase in graphene
Zhang, Y., Tan, Y.-W., Stormer, H. L., & Kim, P. (2005) · Nature · doi:10.1038/nature04235 · Cited by 13,435
Graphene-based nanomaterials and their electrochemistry
Pumera, M. (2010) · Chemical Society Reviews · doi:10.1039/c002690p · Cited by 1,117
Cited by
Wang, J., Liu, J., Chao, D., Yan, J., Lin, J., & Shen, Z. X. (2014) · Advanced Materials · doi:10.1002/adma.201402728 · Cited by 442
Multivalent metal ion hybrid capacitors: a review with a focus on zinc-ion hybrid capacitors
Dong, L., Yang, W., Yang, W., Li, Y., Wu, W., & Wang, G. (2019) · Journal of Materials Chemistry A · doi:10.1039/c9ta02678a · Cited by 438
Carbon-based functional nanomaterials: Preparation, properties and applications
Li, Z., Wang, L., Li, Y., Feng, Y., & Feng, W. (2019) · Composites Science and Technology · doi:10.1016/j.compscitech.2019.04.028 · Cited by 384
Metadata
- Authors
- Fan, W., Zhang, C., Tjiu, W. W., Pramoda, K. P., He, C., & Liu, T.
- Venue
- ACS Applied Materials & Interfaces
- Publisher
- American Chemical Society (ACS)
- Published
- 2013-04-08
- Volume
- 5
- Issue
- 8
- Pages
- 3382-3391
- ISSN
- 1944-8244 (ISSN-L)
- 1944-8252
- OpenAlex
- W1981587003
- Cited by
- 339
- References
- 2
- FWCI
- 13.54
- Type
- journal article
- Language
- en
- Open access
- closed
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- Fan, W., Zhang, C., Tjiu, W. W., Pramoda, K. P., He, C., & Liu, T. (2013). Graphene-Wrapped Polyaniline Hollow Spheres As Novel Hybrid Electrode Materials for Supercapacitor Applications. ACS Applied Materials & Interfaces. https://doi.org/10.1021/am4003827
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