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Synthesis of Magnetically Separable Ag3PO4/TiO2/Fe3O4 Heterostructure with Enhanced Photocatalytic Performance under Visible Light for Photoinactivation of Bacteria
Abstract
Silver orthophosphate (Ag3PO4) is a low-band-gap photocatalyst that has received considerable research interest in recent years. In this work, the magnetic Ag3PO4/TiO2/Fe3O4 heterostructured nanocomposite was synthesized. The nanocomposite was found to exhibit markedly enhanced photocatalytic activity, cycling stability, and long-term durability in the photodegradation of acid orange 7 (AO7) under visible light. Moreover, the antibacterial film prepared from Ag3PO4/TiO2/Fe3O4 nanocomposite presented excellent bactericidal activity and recyclability toward Escherichia coli (E. coli) cells under visible-light irradiation. In addition to the intrinsic cytotoxicity of silver ions, the elevated bactericidal efficiency of Ag3PO4/TiO2/Fe3O4 can be largely attributed to its highly enhanced photocatalytic activity. The photogenerated hydroxyl radicals and superoxide ions on the formed Ag/Ag3PO4/TiO2 interfaces cause considerable morphological changes in the microorganism's cells and lead to the death of the bacteria.
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Cites
Photocatalysis on TiO2 Surfaces: Principles, Mechanisms, and Selected Results
Linsebigler, A. L., Lu, G., & Yates, J. T. (1995) · Chemical Reviews · doi:10.1021/cr00035a013 · Cited by 11,575
Semiconductor-based Photocatalytic Hydrogen Generation
Chen, X., Shen, S., Guo, L., & Mao, S. S. (2010) · Chemical Reviews · doi:10.1021/cr1001645 · Cited by 7,876
Cited by
Efficient visible driven photocatalyst, silver phosphate: performance, understanding and perspective
Martin, D. J., Liu, G., Moniz, S. J. A., Bi, Y., Beale, A. M., Ye, J., & Tang, J. (2015) · Chemical Society Reviews · doi:10.1039/c5cs00380f · Cited by 477
Su, C. (2017) · Journal of Hazardous Materials · doi:10.1016/j.jhazmat.2016.06.060 · Cited by 365
Solar photocatalytic abatement of sulfamethoxazole over Ag3PO4/WO3 composites
Grilla, E., Petala, A., Frontistis, Z., Konstantinou, I. K., Kondarides, D. I., & Mantzavinos, D. (2018) · Applied Catalysis B: Environmental · doi:10.1016/j.apcatb.2018.03.011 · Cited by 85
Metadata
- Authors
- Xu, J.-W., Gao, Z.-D., Han, K., Liu, Y., & Song, Y.-Y.
- Venue
- ACS Applied Materials & Interfaces
- Publisher
- American Chemical Society (ACS)
- Published
- 2014-08-27
- Volume
- 6
- Issue
- 17
- Pages
- 15122-15131
- ISSN
- 1944-8244 (ISSN-L)
- 1944-8252
- OpenAlex
- W2314211852
- Cited by
- 219
- References
- 2
- FWCI
- 8.19
- Type
- journal article
- Language
- en
- Open access
- closed
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- Xu, J.-W., Gao, Z.-D., Han, K., Liu, Y., & Song, Y.-Y. (2014). Synthesis of Magnetically Separable Ag3PO4/TiO2/Fe3O4 Heterostructure with Enhanced Photocatalytic Performance under Visible Light for Photoinactivation of Bacteria. ACS Applied Materials & Interfaces. https://doi.org/10.1021/am5032727
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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