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Construction of Heterostructured g-C3N4/Ag/TiO2 Microspheres with Enhanced Photocatalysis Performance under Visible-Light Irradiation
Abstract
The visible-light photocatalytic performance of the heterostructured g-C3N4/Ag/TiO2 microspheres was investigated. As an electron-conduction bridge, Ag nanoparticles were photodeposited as the interlayer between g-C3N4 and the surface of TiO2 microspheres to increase visible-light absorption via the surface plasmon resonance. The interface between Ag/TiO2 and g-C3N4 facilitates the direct migration of photoinduced electrons from g-C3N4 to Ag/TiO2, which is conductive to retarding the recombination of electron-holes. The g-C3N4 (4%)/Ag/TiO2 microsphere sample shows significant photocatalytic activity, higher than the sum of g-C3N4 (1.2 mg) and Ag/TiO2 samples, or the sum of TiO2 and Ag/g-C3N4 (1.8 mg) samples. It indicates that the heterostructured combination of g-C3N4, Ag and TiO2 microspheres provides synergistic photocatalytic activity through an efficient electron transfer process.
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Cited by
Ong, W.-J., Tan, L.-L., Ng, Y. H., Yong, S.-T., & Chai, S.-P. (2016) · Chemical Reviews · doi:10.1021/acs.chemrev.6b00075 · Cited by 7,147
Hao, R., Wang, G., Tang, H., Sun, L., Xu, C., & Han, D. (2016) · Applied Catalysis B: Environmental · doi:10.1016/j.apcatb.2016.01.026 · Cited by 668
Tong, Z., Yang, D., Shi, J., Nan, Y., Sun, Y., & Jiang, Z. (2015) · ACS Applied Materials & Interfaces · doi:10.1021/acsami.5b09503 · Cited by 431
Chen, F., Yang, Q., Wang, Y., Zhao, J., Wang, D., Li, X., Guo, Z., Wang, H., Deng, Y., Niu, C., et al. (2017) · Applied Catalysis B: Environmental · doi:10.1016/j.apcatb.2016.12.017 · Cited by 429
Emerging Cocatalysts on g‐C3N4 for Photocatalytic Hydrogen Evolution
Zhu, Q., Xu, Z., Qiu, B., Xing, M., & Zhang, J. (2021) · Small · doi:10.1002/smll.202101070 · Cited by 380
Metadata
- Authors
- Chen, Y., Huang, W., He, D., Situ, Y., & Huang, H.
- Venue
- ACS Applied Materials & Interfaces
- Publisher
- American Chemical Society (ACS)
- Published
- 2014-08-11
- Volume
- 6
- Issue
- 16
- Pages
- 14405-14414
- ISSN
- 1944-8244 (ISSN-L)
- 1944-8252
- OpenAlex
- W2318286541
- Cited by
- 693
- References
- 0
- FWCI
- 19.98
- Type
- journal article
- Language
- en
- Open access
- closed
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- Chen, Y., Huang, W., He, D., Situ, Y., & Huang, H. (2014). Construction of Heterostructured g-C3N4/Ag/TiO2 Microspheres with Enhanced Photocatalysis Performance under Visible-Light Irradiation. ACS Applied Materials & Interfaces. https://doi.org/10.1021/am503674e
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