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Fabrication of Multiple Heterojunctions with Tunable Visible-Light-Active Photocatalytic Reactivity in BiOBr–BiOI Full-Range Composites Based on Microstructure Modulation and Band Structures
Abstract
The fabrication of multiple heterojunctions with tunable photocatalytic reactivity in full-range BiOBr-BiOI composites based on microstructure modulation and band structures is demonstrated. The multiple heterojunctions are constructed by precipitation at room temperature and characterized systematically. Photocatalytic experiments indicate that there are two types of heterostructures with distinct photocatalytic mechanisms, both of which can greatly enhance the visible-light photocatalytic performance for the decomposition of organic pollutants and generation of photocurrent. The large separation and inhibited recombination of electron-hole pairs rendered by the heterostructures are confirmed by electrochemical impedance spectra (EIS) and photoluminescence (PL). Reactive species trapping, nitroblue tetrazolium (NBT, detection agent of (•)O2(-)) transformation, and terephthalic acid photoluminescence (TA-PL) experiments verify the charge-transfer mechanism derived from the two types of heterostructures, as well as different enhancements of the photocatalytic activity. This article provides insights into heterostructure photocatalysis and describes a novel way to design and fabricate high-performance semiconductor composites.
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Cites
Generalized Gradient Approximation Made Simple
Perdew, J. P., Burke, K., & Ernzerhof, M. (1996) · Physical Review Letters · doi:10.1103/physrevlett.77.3865 · Cited by 215,824
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Generation and Detection of Reactive Oxygen Species in Photocatalysis
Nosaka, Y., & Nosaka, A. Y. (2017) · Chemical Reviews · doi:10.1021/acs.chemrev.7b00161 · Cited by 4,771
Chen, F., Huang, G.-X., Yao, F.-B., Yang, Q., Zheng, Y.-M., Zhao, Q.-B., & Yu, H.-Q. (2020) · Water Research · doi:10.1016/j.watres.2020.115559 · Cited by 459
Chlorine intercalation in graphitic carbon nitride for efficient photocatalysis
Liu, C., Zhang, Y., Dong, F., Reshak, A. H., Ye, L., Pinna, N., Zeng, C., Zhang, T., & Huang, H. (2017) · Applied Catalysis B: Environmental · doi:10.1016/j.apcatb.2016.10.002 · Cited by 396
Self-citationJiang, X.-H., Xing, Q.-J., Luo, X.-B., Li, F., Zou, J.-P., Liu, S.-S., Li, X., & Wang, X.-K. (2018) · Applied Catalysis B: Environmental · doi:10.1016/j.apcatb.2018.01.062 · Cited by 361
Self-citationDi, J., Xia, J., Ji, M., Wang, B., Yin, S., Zhang, Q., Chen, Z., & Li, H. (2016) · Applied Catalysis B: Environmental · doi:10.1016/j.apcatb.2015.10.036 · Cited by 347
Gao, K., Hou, L.-A., An, X., Huang, D., & Yang, Y. (2023) · Applied Catalysis B: Environmental · doi:10.1016/j.apcatb.2022.122150 · Cited by 270
Metadata
- Authors
- Huang, H., Han, X., Li, X., Wang, S., Chu, P. K., & Zhang, Y.
- Venue
- ACS Applied Materials & Interfaces
- Publisher
- American Chemical Society (ACS)
- Published
- 2015-01-06
- Volume
- 7
- Issue
- 1
- Pages
- 482-492
- ISSN
- 1944-8244 (ISSN-L)
- 1944-8252
- OpenAlex
- W2328859466
- Cited by
- 728
- References
- 1
- FWCI
- 22.92
- Type
- journal article
- Language
- en
- Open access
- closed
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