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Orientational Dynamics of Liquids Confined in Nanoporous Sol−Gel Glasses Studied by Optical Kerr Effect Spectroscopy
Abstract
When a liquid is restricted to volumes on a molecular distance scale, its orientational and translational dynamics are perturbed strongly by the confinement. Nanoporous sol-gel glasses are an excellent model system for studying the effects of confinement on the behavior of liquids, and in this Account we review experiments in which ultrafast optical Kerr effect spectroscopy has been used to study the orientational dynamics of liquids confined in these media. We contrast the effects of confinement on the orientational dynamics of weakly wetting, strongly wetting, and networked liquids, and we discuss the influence of factors such as pore size, molecular shape, and surface chemistry.
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Citations
Cited by
Coherent Two-Dimensional Optical Spectroscopy
Cho, M. (2008) · Chemical Reviews · doi:10.1021/cr078377b · Cited by 835
Critical Knowledge Gaps in Mass Transport through Single-Digit Nanopores: A Review and Perspective
Faucher, S., Aluru, N., Bazant, M. Z., Blankschtein, D., Brozena, A. H., Cumings, J., Pedro de Souza, J., Elimelech, M., Epsztein, R., Fourkas, J. T., et al. (2019) · The Journal of Physical Chemistry C · doi:10.1021/acs.jpcc.9b02178 · Cited by 365
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Metadata
- Authors
- Farrer, R. A., & Fourkas, J. T.
- Venue
- Accounts of Chemical Research
- Publisher
- American Chemical Society (ACS)
- Published
- 2003-05-07
- Volume
- 36
- Issue
- 8
- Pages
- 605-612
- ISSN
- 0001-4842 (ISSN-L)
- 1520-4898
- OpenAlex
- W2073690435
- Cited by
- 182
- References
- 0
- FWCI
- 5.93
- Type
- journal article
- Language
- en
- Open access
- closed
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- Farrer, R. A., & Fourkas, J. T. (2003). Orientational Dynamics of Liquids Confined in Nanoporous Sol−Gel Glasses Studied by Optical Kerr Effect Spectroscopy. Accounts of Chemical Research. https://doi.org/10.1021/ar0200302
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