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Mesoporous Tantalum Oxide. 1. Characterization and Photocatalytic Activity for the Overall Water Decomposition
Abstract
Mesoporous Ta 2 O 5 was synthesized by the ligand-assisted templating method, and its stability for use as a photocatalyst was studied by X-ray diffraction, N 2 adsorption isotherm analysis, and transmission electron microscopy. The photocatalytic activity for the overall water decomposition on the mesoporous Ta 2 O 5 was improved by NiO loading and pretreatment. The mesoporous structure was found to be maintained to some extent after loading of NiO (H 2 evolution site) and pretreatment for activation at a temperature as high as 673 K. Although the wall of mesoporous Ta 2 O 5 was amorphous, the photocatalytic activity was higher than that of the crystallized Ta 2 O 5 .
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Cites
Generalized syntheses of large-pore mesoporous metal oxides with semicrystalline frameworks
Yang, P., Zhao, D., Margolese, D. I., Chmelka, B. F., & Stucky, G. D. (1998) · Nature · doi:10.1038/24132 · Cited by 2,493
Cited by
Semiconductor-based Photocatalytic Hydrogen Generation
Chen, X., Shen, S., Guo, L., & Mao, S. S. (2010) · Chemical Reviews · doi:10.1021/cr1001645 · Cited by 7,876
Ordered mesoporous materials in catalysis
Taguchi, A., & Schüth, F. (2005) · Microporous and Mesoporous Materials · doi:10.1016/j.micromeso.2004.06.030 · Cited by 2,119
Nanostructured materials for photocatalysis
Xu, C., Ravi Anusuyadevi, P., Aymonier, C., Luque, R., & Marre, S. (2019) · Chemical Society Reviews · doi:10.1039/c9cs00102f · Cited by 1,082
Tantalum-based semiconductors for solar water splitting
Zhang, P., Zhang, J., & Gong, J. (2014) · Chem. Soc. Rev. · doi:10.1039/c3cs60438a · Cited by 494
Metadata
- Authors
- Takahara, Y., Kondo, J. N., Takata, T., Lu, D., & Domen, K.
- Venue
- Chemistry of Materials
- Publisher
- American Chemical Society (ACS)
- Published
- 2001-03-07
- Volume
- 13
- Issue
- 4
- Pages
- 1194-1199
- ISSN
- 0897-4756 (ISSN-L)
- 1520-5002
- OpenAlex
- W1969314523
- Cited by
- 234
- References
- 1
- FWCI
- 8.83
- Type
- journal article
- Language
- en
- Open access
- closed
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- Takahara, Y., Kondo, J. N., Takata, T., Lu, D., & Domen, K. (2001). Mesoporous Tantalum Oxide. 1. Characterization and Photocatalytic Activity for the Overall Water Decomposition. Chemistry of Materials. https://doi.org/10.1021/cm000572i
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