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Pseudocapacitive Lithium Storage in TiO2(B)
Open accessAbstract
Phase-pure TiO 2 (B) with microfibrous morphology was prepared via a newly developed method from amorphous TiO 2 . Cyclic voltammetry evidences that Li-insertion into TiO 2 (B) is governed by a pseudocapacitive faradaic process, whose rate is not limited by solid-state diffusion of Li + in a broad interval of scan rates. This unusual behavior was discussed in terms of the crystal structure of the TiO 2 (B) host, having freely accessible parallel channels for Li + -transport perpendicular to the (010) face. The characteristic Li-insertion electrochemistry of TiO 2 (B) allows re-interpretation of several previous reports, which did not consider explicitly this relation or the presence of TiO 2 (B) in various TiO 2 materials of different origin.
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Cited by
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Brezesinski, T., Wang, J., Tolbert, S. H., & Dunn, B. (2010) · Nature Materials · doi:10.1038/nmat2612 · Cited by 3,359
Achieving high energy density and high power density with pseudocapacitive materials
Choi, C., Ashby, D. S., Butts, D. M., DeBlock, R. H., Wei, Q., Lau, J., & Dunn, B. (2019) · Nature Reviews Materials · doi:10.1038/s41578-019-0142-z · Cited by 1,964
Advanced Energy Storage Devices: Basic Principles, Analytical Methods, and Rational Materials Design
Liu, J., Wang, J., Xu, C., Jiang, H., Li, C., Zhang, L., Lin, J., & Shen, Z. X. (2018) · Advanced Science · doi:10.1002/advs.201700322 · Cited by 1,745
Protonated Titanates and TiO2 Nanostructured Materials: Synthesis, Properties, and Applications
Bavykin, D. V., Friedrich, J. M., & Walsh, F. C. (2006) · Advanced Materials · doi:10.1002/adma.200502696 · Cited by 1,634
Chodankar, N. R., Pham, H. D., Nanjundan, A. K., Fernando, J. F. S., Jayaramulu, K., Golberg, D., Han, Y., & Dubal, D. P. (2020) · Small · doi:10.1002/smll.202002806 · Cited by 852
Metadata
- Authors
- Zukalová, M., Kalbáč, M., Kavan, L., Exnar, I., & Graetzel, M.
- Venue
- Chemistry of Materials
- Publisher
- American Chemical Society (ACS)
- Published
- 2005-02-08
- Volume
- 17
- Issue
- 5
- Pages
- 1248-1255
- ISSN
- 0897-4756 (ISSN-L)
- 1520-5002
- OpenAlex
- W2109593963
- Cited by
- 500
- References
- 0
- FWCI
- 10.80
- Type
- journal article
- Language
- en
- Open access
- green
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- Zukalová, M., Kalbáč, M., Kavan, L., Exnar, I., & Graetzel, M. (2005). Pseudocapacitive Lithium Storage in TiO2(B). Chemistry of Materials. https://doi.org/10.1021/cm048249t
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