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Acid-Catalyzed Reactions on Flexible Polycyclic Aromatic Carbon in Amorphous Carbon
Abstract
Carbonization of d -glucose at 573−723 K followed by sulfonation produces a functionalized amorphous carbon material with acid catalytic activity as a solid-acid replacement for sulfuric acid. The carbon material contains phenolic hydroxyl, carboxylic acid, and sulfonic acid groups and exhibits high catalytic performance for liquid-phase acid-catalyzed reactions. Carbonization at higher temperature followed by sulfonation also results in amorphous carbon, but the resultant does not exhibit catalytic activity although the amorphous carbon has sufficient amount of sulfonic acid groups. Structural and active site analyses suggest that the marked difference in catalytic activity is due to the accessibility of reactants to sulfonic acid groups in the carbon structure.
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Cited by
Development of biochar-based functional materials: toward a sustainable platform carbon material
Liu, W.-J., Jiang, H., & Yu, H.-Q. (2015) · Chemical Reviews · doi:10.1021/acs.chemrev.5b00195 · Cited by 1,754
Hydrolysis of Cellulose by Amorphous Carbon Bearing SO3H, COOH, and OH Groups
Suganuma, S., Nakajima, K., Kitano, M., Yamaguchi, D., Kato, H., Hayashi, S., & Hara, M. (2008) · Journal of the American Chemical Society · doi:10.1021/ja803983h · Cited by 1,020
Self-citationLee, J., Kim, K.-H., & Kwon, E. E. (2017) · Renewable and Sustainable Energy Reviews · doi:10.1016/j.rser.2017.04.002 · Cited by 668
Amorphous Carbon with SO3H Groups as a Solid Brønsted Acid Catalyst
Nakajima, K., & Hara, M. (2012) · ACS Catalysis · doi:10.1021/cs300103k · Cited by 435
Self-citationSO 3 H-Containing Functional Carbon Materials: Synthesis, Structure, and Acid Catalysis
Konwar, L. J., Mäki-Arvela, P., & Mikkola, J.-P. (2019) · Chemical Reviews · doi:10.1021/acs.chemrev.9b00199 · Cited by 305
Metadata
- Authors
- Okamura, M., Takagaki, A., Toda, M., Kondo, J. N., Domen, K., Tatsumi, T., Hara, M., & Hayashi, S.
- Venue
- Chemistry of Materials
- Publisher
- American Chemical Society (ACS)
- Published
- 2006-06-01
- Volume
- 18
- Issue
- 13
- Pages
- 3039-3045
- ISSN
- 0897-4756 (ISSN-L)
- 1520-5002
- OpenAlex
- W2009094440
- Cited by
- 570
- References
- 0
- FWCI
- 7.81
- Type
- journal article
- Language
- en
- Open access
- closed
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- Okamura, M., Takagaki, A., Toda, M., Kondo, J. N., Domen, K., Tatsumi, T., Hara, M., & Hayashi, S. (2006). Acid-Catalyzed Reactions on Flexible Polycyclic Aromatic Carbon in Amorphous Carbon. Chemistry of Materials. https://doi.org/10.1021/cm0605623
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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