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Highly Electrochemical Reaction of Lithium in the Ordered Mesoporosus β-MnO2
Abstract
The highly crystallized β-MnO 2 with the narrowest [1 × 1] channels prepared by direct thermal decomposition of Mn(NO 3 ) 2 does not provide much capacity due to the poor kinetics of the lithium intercalation/deintercalation process. In the present work, we report the preparation and electrochemical performance of an ordered mesoporous β-MnO 2 as a positive electrode for rechargeable lithium batteries. The well-ordered mesoporous β-MnO 2 prepared using mesoporous silica KIT-6 as a template by thermal decomposition of Mn(NO 3 ) 2 exhibits high initial capacity, reaching a chemical composition of Li 0.75 MnO 2, and it also shows a good rate capability and cycling ability. The correlation between the specific mesoporous structure and the superior electrochemical performance was discussed in detail.
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Cited by
Ordered mesoporous metal oxides: synthesis and applications
Ren, Y., Ma, Z., & Bruce, P. G. (2012) · Chemical Society Reviews · doi:10.1039/c2cs35086f · Cited by 768
Porous electrode materials for lithium-ion batteries–how to prepare them and what makes them special
Vu, A., Qian, Y., & Stein, A. (2012) · Advanced Energy Materials · doi:10.1002/aenm.201200320 · Cited by 719
Synthesis of non-siliceous mesoporous oxides
Gu, D., & Schüth, F. (2014) · Chem. Soc. Rev. · doi:10.1039/c3cs60155b · Cited by 584
Template-Directed Materials for Rechargeable Lithium-Ion Batteries
Cheng, F., Tao, Z., Liang, J., & Chen, J. (2008) · Chemistry of Materials · doi:10.1021/cm702091q · Cited by 537
Layered lithium transition metal oxide cathodes towards high energy lithium-ion batteries
He, P., Yu, H., Li, D., & Zhou, H. (2012) · Journal of Materials Chemistry · doi:10.1039/c2jm14305d · Cited by 472
Metadata
- Authors
- Luo, J.-Y., Zhang, J.-J., & Xia, Y.-Y.
- Venue
- Chemistry of Materials
- Publisher
- American Chemical Society (ACS)
- Published
- 2006-10-14
- Volume
- 18
- Issue
- 23
- Pages
- 5618-5623
- ISSN
- 0897-4756 (ISSN-L)
- 1520-5002
- OpenAlex
- W2952290842
- Cited by
- 189
- References
- 0
- FWCI
- 13.50
- Type
- journal article
- Language
- en
- Open access
- closed
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- Luo, J.-Y., Zhang, J.-J., & Xia, Y.-Y. (2006). Highly Electrochemical Reaction of Lithium in the Ordered Mesoporosus β-MnO2. Chemistry of Materials. https://doi.org/10.1021/cm061458o
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