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Selective Growth and MOCVD Loading of Small Single Crystals of MOF-5 at Alumina and Silica Surfaces Modified with Organic Self-Assembled Monolayers
Abstract
Thin polycrystalline films of phase-pure MOF-5 were grown directly from supersaturated MOF-5 mother solutions on suitably pretreated alumina and silica substrates. The surface acid/base properties characterized by the isoelectric point of the bare substrates controls the anchoring of MOF-5 nuclei. In addition to COOH-terminated SAMs on SiO 2, ALD-Al 2 O 3 proved to be a very good adhesive for selective MOF-5 growth. The adsorption properties of the deposited MOF films on Al 2 O 3 substrates were demonstrated by MOCVD loading with [(η 5 -C 5 H 5 )Pd(η 3 -C 3 H 5 )] as Pd precursor to finally yield the palladium-loaded thin film material {Pd@MOF-5}/Al 2 O 3 as a model of a variety of conceivable MOF-based functional chemical systems at surfaces.
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Cites
Amorphous Calcium Carbonate: Synthesis and Potential Intermediate in Biomineralization
Faatz, M., Gröhn, F., & Wegner, G. (2004) · Advanced Materials · doi:10.1002/adma.200306565 · Cited by 343
Cited by
Thin films of metal–organic frameworks
Zacher, D., Shekhah, O., Wöll, C., & Fischer, R. A. (2009) · Chemical Society Reviews · doi:10.1039/b805038b · Cited by 893
Self-citationMetal–organic frameworks for membrane-based separations
Denny, M. S., Moreton, J. C., Benz, L., & Cohen, S. M. (2016) · Nature Reviews Materials · doi:10.1038/natrevmats.2016.78 · Cited by 820
MOF positioning technology and device fabrication
Falcaro, P., Ricco, R., Doherty, C. M., Liang, K., Hill, A. J., & Styles, M. J. (2014) · Chem. Soc. Rev. · doi:10.1039/c4cs00089g · Cited by 710
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Ahmed, I., & Jhung, S. H. (2014) · Materials Today · doi:10.1016/j.mattod.2014.03.002 · Cited by 451
Manufacture of dense coatings of Cu3(BTC)2 (HKUST-1) on α-alumina
Gascon, J., Aguado, S., & Kapteijn, F. (2008) · Microporous and Mesoporous Materials · doi:10.1016/j.micromeso.2007.11.014 · Cited by 334
Metadata
- Authors
- Hermes, S., Zacher, D., Baunemann, A., Wöll, C., & Fischer, R. A.
- Venue
- Chemistry of Materials
- Publisher
- American Chemical Society (ACS)
- Published
- 2007-04-07
- Volume
- 19
- Issue
- 9
- Pages
- 2168-2173
- ISSN
- 0897-4756 (ISSN-L)
- 1520-5002
- OpenAlex
- W2088260361
- Cited by
- 184
- References
- 1
- FWCI
- 10.02
- Type
- journal article
- Language
- en
- Open access
- closed
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- Hermes, S., Zacher, D., Baunemann, A., Wöll, C., & Fischer, R. A. (2007). Selective Growth and MOCVD Loading of Small Single Crystals of MOF-5 at Alumina and Silica Surfaces Modified with Organic Self-Assembled Monolayers. Chemistry of Materials. https://doi.org/10.1021/cm062854%2B
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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