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Structure and Electrochemistry of Copper Fluoride Nanocomposites Utilizing Mixed Conducting Matrices
Abstract
Near-theoretical utilization of high-energy-density CuF 2 positive electrode materials for lithium batteries was enabled through the use of nanocomposites consisting of 2−30 nm domains of CuF 2 within a mixed ionic + electronic conducting matrix of a metal oxide. Small but significant crystallographic changes to the core crystal of the CuF 2 were found to occur in all oxide-based matrices. These modifications to the core crystal and the surrounding matrix were investigated through a host of characterization methods, including XRD, XPS, and XAS. This new approach to the enablement of the anhydrous CuF 2 is distinctly superior in performance to that of macro CuF 2 or CuF 2 nanocomposites utilizing carbon as a matrix, the latter of which is also introduced herein for the first time.
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Cited by
Cabana, J., Monconduit, L., Larcher, D., & Palacín, M. R. (2010) · Advanced Materials · doi:10.1002/adma.201000717 · Cited by 2,361
Coaxial MnO2/Carbon Nanotube Array Electrodes for High-Performance Lithium Batteries
Reddy, A. L. M., Shaijumon, M. M., Gowda, S. R., & Ajayan, P. M. (2009) · Nano Letters · doi:10.1021/nl803081j · Cited by 962
Electrode Degradation in Lithium-Ion Batteries
Pender, J. P., Jha, G., Youn, D. H., Ziegler, J. M., Andoni, I., Choi, E. J., Heller, A., Dunn, B. S., Weiss, P. S., Penner, R. M., et al. (2020) · ACS Nano · doi:10.1021/acsnano.9b04365 · Cited by 873
Hybrid supercapacitor-battery materials for fast electrochemical charge storage
Vlad, A., Singh, N., Rolland, J., Melinte, S., Ajayan, P. M., & Gohy, J.-F. (2014) · Scientific Reports · doi:10.1038/srep04315 · Cited by 334
Nanoscale Phenomena in Lithium-Ion Batteries
Jung, S.-K., Hwang, I., Chang, D., Park, K.-Y., Kim, S. J., Seong, W. M., Eum, D., Park, J., Kim, B., Kim, J., et al. (2020) · Chemical Reviews · doi:10.1021/acs.chemrev.9b00405 · Cited by 253
Metadata
- Authors
- Badway, F., Mansour, A. N., Pereira, N., Al-Sharab, J. F., Cosandey, F., Plitz, I., & Amatucci, G. G.
- Venue
- Chemistry of Materials
- Publisher
- American Chemical Society (ACS)
- Published
- 2007-07-21
- Volume
- 19
- Issue
- 17
- Pages
- 4129-4141
- ISSN
- 0897-4756 (ISSN-L)
- 1520-5002
- OpenAlex
- W2063139960
- Cited by
- 185
- References
- 0
- FWCI
- 9.13
- Type
- journal article
- Language
- en
- Open access
- closed
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- Badway, F., Mansour, A. N., Pereira, N., Al-Sharab, J. F., Cosandey, F., Plitz, I., & Amatucci, G. G. (2007). Structure and Electrochemistry of Copper Fluoride Nanocomposites Utilizing Mixed Conducting Matrices. Chemistry of Materials. https://doi.org/10.1021/cm070421g
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