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Thermal Behavior of Methylammonium Lead-Trihalide Perovskite Photovoltaic Light Harvesters
Open accessAbstract
Recently organic–inorganic hybrid perovskites have attracted attention as light harvesting materials in mesoscopic cells. While a considerable number of deposition and formation methods have been reported for the perovskite crystalline material, most involve an annealing step. As such, the thermal behavior of this material and its individual components is of crucial interest. Here, we examine the thermal properties of the CH 3 NH 3 PbX 3 (X = I or Cl) perovskite using thermogravimetric analysis. The role of the precursors is exposed, and the effect of the formation of excess organic species is investigated. The sublimation behavior of the organic component is intensively scrutinized. Furthermore, differential scanning calorimetry is employed to probe the crystal phase structure, revealing subtle differences depending on the deposition method.
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Citations
Cited by
Improving the Stability of Metal Halide Perovskite Materials and Light‐Emitting Diodes
Cho, H., Kim, Y., Wolf, C., Lee, H., & Lee, T. (2018) · Advanced Materials · doi:10.1002/adma.201704587 · Cited by 470
Device stability of perovskite solar cells – A review
Asghar, M. I., Zhang, J., Wang, H., & Lund, P. D. (2017) · Renewable and Sustainable Energy Reviews · doi:10.1016/j.rser.2017.04.003 · Cited by 423
Palazon, F., Akkerman, Q. A., Prato, M., & Manna, L. (2016) · ACS Nano · doi:10.1021/acsnano.5b06536 · Cited by 369
Chiba, T., Hoshi, K., Pu, Y.-J., Takeda, Y., Hayashi, Y., Ohisa, S., Kawata, S., & Kido, J. (2017) · ACS Applied Materials & Interfaces · doi:10.1021/acsami.7b03382 · Cited by 336
Song, Z., Watthage, S. C., Phillips, A. B., Tompkins, B. L., Ellingson, R. J., & Heben, M. J. (2015) · Chemistry of Materials · doi:10.1021/acs.chemmater.5b01017 · Cited by 258
Metadata
- Authors
- Dualeh, A., Gao, P., Seok, S. I., Nazeeruddin, M. K., & Grätzel, M.
- Venue
- Chemistry of Materials
- Publisher
- American Chemical Society (ACS)
- Published
- 2014-10-29
- Volume
- 26
- Issue
- 21
- Pages
- 6160-6164
- ISSN
- 0897-4756 (ISSN-L)
- 1520-5002
- OpenAlex
- W2008106023
- Cited by
- 574
- References
- 0
- FWCI
- 30.95
- Type
- journal article
- Language
- en
- Open access
- green
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- Dualeh, A., Gao, P., Seok, S. I., Nazeeruddin, M. K., & Grätzel, M. (2014). Thermal Behavior of Methylammonium Lead-Trihalide Perovskite Photovoltaic Light Harvesters. Chemistry of Materials. https://doi.org/10.1021/cm502468k
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