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Stability of Surface-Immobilized Lubricant Interfaces under Flow
Open accessAbstract
The stability and longevity of surface-stabilized lubricant layers is a critical question in their application as low- and nonfouling slippery surface treatments in both industry and medicine. Here, we investigate lubricant loss from surfaces under flow in water using both quantitative analysis and visualization, testing the effects of underlying surface type (nanostructured versus flat), as well as flow rate in the physiologically relevant range, lubricant type, and time. We find lubricant losses on the order of only ng/cm 2 in a closed system, indicating that these interfaces are relatively stable under the flow conditions tested. No notable differences emerged between surface type, flow rate, lubricant type, or time. However, exposure of the lubricant layers to an air/water interface did significantly increase the amount of lubricant removed from the surface, leading to disruption of the layer. These results may help in the development and design of materials using surface-immobilized lubricant interfaces for repellency under flow conditions.
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Citations
Cites
Liquid-Infused Nanostructured Surfaces with Extreme Anti-Ice and Anti-Frost Performance
Kim, P., Wong, T.-S., Alvarenga, J., Kreder, M. J., Adorno-Martinez, W. E., & Aizenberg, J. (2012) · ACS Nano · doi:10.1021/nn302310q · Cited by 1,316
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Liquid-Infused Surfaces: A Review of Theory, Design, and Applications
Villegas, M., Zhang, Y., Abu Jarad, N., Soleymani, L., & Didar, T. F. (2019) · ACS Nano · doi:10.1021/acsnano.9b04129 · Cited by 459
Peppou-Chapman, S., Hong, J. K., Waterhouse, A., & Neto, C. (2020) · Chemical Society Reviews · doi:10.1039/d0cs00036a · Cited by 373
Self-citationDesigning Bioinspired Anti‐Biofouling Surfaces based on a Superwettability Strategy
Zhang, P., Lin, L., Zang, D., Guo, X., & Liu, M. (2017) · Small · doi:10.1002/smll.201503334 · Cited by 266
Metadata
- Authors
- Howell, C., Vu, T. L., Johnson, C. P., Hou, X., Ahanotu, O., Alvarenga, J., Leslie, D. C., Uzun, O., Waterhouse, A., Kim, P., Super, M., Aizenberg, M., Ingber, D. E., & Aizenberg, J.
- Venue
- Chemistry of Materials
- Publisher
- American Chemical Society (ACS)
- Published
- 2015-02-20
- Volume
- 27
- Issue
- 5
- Pages
- 1792-1800
- ISSN
- 0897-4756 (ISSN-L)
- 1520-5002
- OpenAlex
- W2074376605
- Cited by
- 232
- References
- 1
- FWCI
- 7.55
- Type
- journal article
- Language
- en
- Open access
- green
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- Howell, C., Vu, T. L., Johnson, C. P., Hou, X., Ahanotu, O., Alvarenga, J., Leslie, D. C., Uzun, O., Waterhouse, A., Kim, P., Super, M., Aizenberg, M., Ingber, D. E., & Aizenberg, J. (2015). Stability of Surface-Immobilized Lubricant Interfaces under Flow. Chemistry of Materials. https://doi.org/10.1021/cm504652g
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