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Coordination Networks Based on Multitopic Ligands and Silver(I) Salts: A Study of Network Connectivity and Topology as a Function of Counterion
Abstract
We show that much like hydrogen bonding, Ag−N coordination bonds can be reliably used for the construction of supramolecular networks. From a solid-state structural study of silver(I) complexes of multitopic ligands, we describe coordination networks formed in the presence of the weakly coordinating triflate (CF 3 SO 3 - ) counterion and the noncoordinating hexafluorophosphate (PF 6 - ) species. For complexes prepared with silver(I) triflate, counterion coordination is characteristic. Also, for the triflate complexes presented, ditopic ligands form one-dimensional, chainlike structures and tritopic ligands form 3-connected nets. A tetratopic ligand also forms a 3-connected net due to the triflate-capped silver(I) coordination. In contrast, more varied network topology is seen in complexes of ditopic ligands prepared with silver(I) hexafluorophosphate.
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Citations
Cited by
Leong, W. L., & Vittal, J. J. (2011) · Chemical Reviews · doi:10.1021/cr100160e · Cited by 1,113
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Einander durchdringende Netze: geordnete, periodische Verschlingung
Batten, S. R., & Robson, R. (1998) · Angewandte Chemie · doi:10.1002/(sici)1521-3757(19980605)110:11<1558::aid-ange1558>3.0.co;2-7 · Cited by 466
Entangled Two-Dimensional Coordination Networks: A General Survey
Carlucci, L., Ciani, G., Proserpio, D. M., Mitina, T. G., & Blatov, V. A. (2014) · Chemical Reviews · doi:10.1021/cr500150m · Cited by 285
Metadata
- Authors
- Venkataraman, D., Lee, S., Moore, J. S., Zhang, P., Hirsch, K. A., Gardner, G. B., Covey, A. C., & Prentice, C. L.
- Venue
- Chemistry of Materials
- Publisher
- American Chemical Society (ACS)
- Published
- 1996-01-01
- Volume
- 8
- Issue
- 8
- Pages
- 2030-2040
- ISSN
- 0897-4756 (ISSN-L)
- 1520-5002
- OpenAlex
- W2003549165
- Cited by
- 175
- References
- 0
- FWCI
- 8.97
- Type
- journal article
- Language
- en
- Open access
- closed
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