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Quantitative Determination of Organic Semiconductor Microstructure from the Molecular to Device Scale
Abstract
A study was conducted to demonstrate quantitative determination of organic semiconductor microstructure from the molecular to device scale. The quantitative determination of organic semiconductor microstructure from the molecular to device scale was key to obtaining precise description of the molecular structure and microstructure of the materials of interest. This information combined with electrical characterization and modeling allowed for the establishment of general design rules to guide future rational design of materials and devices. Investigations revealed that a number and variety of defects were the largest contributors to the existence of disorder within a lattice, as organic semiconductor crystals were dominated by weak van der Waals bonding. Crystallite size, texture, and variations in structure due to spatial confinement and interfaces were also found to be relevant for transport of free charge carriers and bound excitonic species over distances that were important for device operation.
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Cited by
Structural control of mixed ionic and electronic transport in conducting polymers
Rivnay, J., Inal, S., Collins, B. A., Sessolo, M., Stavrinidou, E., Strakosas, X., Tassone, C., Delongchamp, D. M., & Malliaras, G. G. (2016) · Nature Communications · doi:10.1038/ncomms11287 · Cited by 939
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Self-citationKan, B., Feng, H., Wan, X., Liu, F., Ke, X., Wang, Y., Wang, Y., Zhang, H., Li, C., Hou, J., et al. (2017) · Journal of the American Chemical Society · doi:10.1021/jacs.7b01170 · Cited by 474
Koch, F. P. V., Rivnay, J., Foster, S., Müller, C., Downing, J. M., Buchaca-Domingo, E., Westacott, P., Yu, L., Yuan, M., Baklar, M., et al. (2013) · Progress in Polymer Science · doi:10.1016/j.progpolymsci.2013.07.009 · Cited by 337
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Metadata
- Authors
- Rivnay, J., Mannsfeld, S. C. B., Miller, C. E., Salleo, A., & Toney, M. F.
- Venue
- Chemical Reviews
- Publisher
- American Chemical Society (ACS)
- Published
- 2012-08-09
- Volume
- 112
- Issue
- 10
- Pages
- 5488-5519
- ISSN
- 0009-2665 (ISSN-L)
- 1520-6890
- OpenAlex
- W2317506299
- Cited by
- 1,419
- References
- 0
- FWCI
- 6.77
- Type
- journal article
- Language
- en
- Open access
- closed
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- Rivnay, J., Mannsfeld, S. C. B., Miller, C. E., Salleo, A., & Toney, M. F. (2012). Quantitative Determination of Organic Semiconductor Microstructure from the Molecular to Device Scale. Chemical Reviews. https://doi.org/10.1021/cr3001109
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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