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Supported Cobalt Oxide Nanoparticles As Catalyst for Aerobic Oxidation of Alcohols in Liquid Phase

Zhu, Junjiang, Kailasam, Kamalakannan, Fischer, Anna, Thomas, Arne·2011·ACS Catalysis
DOI 10.1021/cs100153a
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Abstract

Supported cobalt oxide nanoparticles (NPs) have been prepared by wetness impregnation on different supports and subsequent heat treatment in argon at 350 °C for 2 h. The thus prepared cobalt oxide (Co 3 O 4 ) can be well dispersed on carbonaceous materials such as activated carbon (AC) and covalent trizaine frameworks (CTF), with average particle sizes below 5 nm. The catalytic performance of supported Co 3 O 4 NPs was tested by aerobic oxidation of alcohols in liquid phase. The results show that AC supported Co 3 O 4 NPs, Co 3 O 4 /AC, exhibit ∼100% conversions for alcohol oxidation and can be reused for at least 4 runs without appreciable loss of activity, when a thermal regeneration step is carried out, suggesting that the Co 3 O 4 NPs are well embedded and stabilized on the support, making Co 3 O 4 /AC a promising catalyst for aerobic oxidation of alcohols in liquid phase.

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Cited by

Metadata

Authors
Zhu, J., Kailasam, K., Fischer, A., & Thomas, A.
Venue
ACS Catalysis
Publisher
American Chemical Society (ACS)
Published
2011-03-02
Volume
1
Issue
4
Pages
342-347
ISSN
2155-5435 (ISSN-L)
DOI
10.1021/cs100153a
OpenAlex
W2317294870
Cited by
206
References
0
FWCI
4.34
Type
journal article
Language
en
Open access
closed

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