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Amine-Functionalized GO as an Active and Reusable Acid–Base Bifunctional Catalyst for One-Pot Cascade Reactions
Abstract
The amine-functionalized graphene oxide was prepared by a facile one-step silylation approach and used as an acid–base bifunctional catalyst in one-pot cascade reactions containing successive acetal hydrolysis and Knoevenagel condensation owing to the separate coexistence of original carboxylic acid on the edge of the GO sheet and the postgrafted amine groups on the GO basal surface. This catalyst exhibited much higher activity than either amine-functionalized active carbon, amine-functionalized SBA-15, or amine-functionalized Al 2 O 3 due to the enriched surface acid sites and the diminished diffusion limitation as well as high catalyst dispersion in liquid solution due to the unique two-dimensional structure. More importantly, this catalyst could be easily recycled and used repetitively, showing potential application in industry.
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Citations
Cites
Nanocrystal Growth on Graphene with Various Degrees of Oxidation
Wang, H., Robinson, J. T., Diankov, G., & Dai, H. (2010) · Journal of the American Chemical Society · doi:10.1021/ja100329d · Cited by 530
Cited by
Zaera, F. (2022) · Chemical Reviews · doi:10.1021/acs.chemrev.1c00905 · Cited by 425
Design and fabrication of mesoporous heterogeneous basic catalysts
Sun, L.-B., Liu, X.-Q., & Zhou, H.-C. (2015) · Chemical Society Reviews · doi:10.1039/c5cs00090d · Cited by 386
Metadata
- Authors
- Zhang, F., Jiang, H., Li, X., Wu, X., & Li, H.
- Venue
- ACS Catalysis
- Publisher
- American Chemical Society (ACS)
- Published
- 2013-12-31
- Volume
- 4
- Issue
- 2
- Pages
- 394-401
- ISSN
- 2155-5435 (ISSN-L)
- OpenAlex
- W2316862897
- Cited by
- 168
- References
- 1
- FWCI
- 6.03
- Type
- journal article
- Language
- en
- Open access
- closed
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- Zhang, F., Jiang, H., Li, X., Wu, X., & Li, H. (2014). Amine-Functionalized GO as an Active and Reusable Acid–Base Bifunctional Catalyst for One-Pot Cascade Reactions. ACS Catalysis. https://doi.org/10.1021/cs400761r
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