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Reusable Homogeneous Catalytic System for Hydrogen Production from Methanol and Water
Abstract
An efficient system catalyzed by a Ru-PNN pincer complex was developed for reforming methanol to H 2 and CO 2 (absorbed by base) under relatively low temperature (around 100 °C), and good yields of H 2 were obtained (∼80%). The catalyst solution can be reused without isolation and purification, with no decrease in catalytic activity being observed for a period of ∼1 month. Decomposition of formic acid, which is likely to be the last step of the methanol reforming reaction, was also investigated, and the formic acid adduct of the catalyst was fully characterized spectroscopically and by X-ray crystallography.
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Cited by
Homogeneous Catalysis for Sustainable Hydrogen Storage in Formic Acid and Alcohols
Sordakis, K., Tang, C., Vogt, L. K., Junge, H., Dyson, P. J., Beller, M., & Laurenczy, G. (2018) · Chemical Reviews · doi:10.1021/acs.chemrev.7b00182 · Cited by 1,110
Bond Activation and Catalysis by Ruthenium Pincer Complexes
Gunanathan, C., & Milstein, D. (2014) · Chemical Reviews · doi:10.1021/cr5002782 · Cited by 958
Self-citationKlankermayer, J., Wesselbaum, S., Beydoun, K., & Leitner, W. (2016) · Angewandte Chemie International Edition · doi:10.1002/anie.201507458 · Cited by 856
Metadata
- Authors
- Hu, P., Diskin-Posner, Y., Ben-David, Y., & Milstein, D.
- Venue
- ACS Catalysis
- Publisher
- American Chemical Society (ACS)
- Published
- 2014-07-10
- Volume
- 4
- Issue
- 8
- Pages
- 2649-2652
- ISSN
- 2155-5435 (ISSN-L)
- OpenAlex
- W2327931639
- Cited by
- 198
- References
- 0
- FWCI
- 9.89
- Type
- journal article
- Language
- en
- Open access
- closed
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Bibliographic data: Semantic Scholar, OpenAlex, Crossref.
Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
