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Degradation Pathways for Monoethanolamine in a CO2 Capture Facility
Abstract
One of the highest priorities in carbon sequestration science is the development of techniques for CO 2 separation and capture, because it is expected to account for the majority of the total cost (∼75%). The most common currently used method of CO 2 separation is reversible chemical absorption using monoethanolamine (MEA) solvent. In the current study, solvent degradation from this technique was studied using degraded MEA samples from the IMC Chemicals Facility in Trona, California. A major pathway to solvent degradation that had not been previously observed in laboratory experiments has been identified. This pathway, which is initiated by oxidation of the solvent, is a much more significant source of solvent degradation than the previously identified carbamate dimerization mechanism.
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Citations
Cited by
CO2 capture and separation technologies for end-of-pipe applications – A review
Olajire, A. A. (2010) · Energy · doi:10.1016/j.energy.2010.02.030 · Cited by 1,217
Air as the renewable carbon source of the future: an overview of CO2 capture from the atmosphere
Goeppert, A., Czaun, M., Surya Prakash, G. K., & Olah, G. A. (2012) · Energy & Environmental Science · doi:10.1039/c2ee21586a · Cited by 724
Carbon-Based Adsorbents for Postcombustion CO 2 Capture: A Critical Review
Creamer, A. E., & Gao, B. (2016) · Environmental Science & Technology · doi:10.1021/acs.est.6b00627 · Cited by 598
Amine degradation in CO2 capture. I. A review
Gouedard, C., Picq, D., Launay, F., & Carrette, P.-L. (2012) · International Journal of Greenhouse Gas Control · doi:10.1016/j.ijggc.2012.06.015 · Cited by 560
Koornneef, J., van Keulen, T., Faaij, A., & Turkenburg, W. (2008) · International Journal of Greenhouse Gas Control · doi:10.1016/j.ijggc.2008.06.008 · Cited by 396
Metadata
- Authors
- Strazisar, B. R., Anderson, R. R., & White, C. M.
- Venue
- Energy & Fuels
- Publisher
- American Chemical Society (ACS)
- Published
- 2003-06-04
- Volume
- 17
- Issue
- 4
- Pages
- 1034-1039
- ISSN
- 0887-0624 (ISSN-L)
- 1520-5029
- OpenAlex
- W2145009485
- Cited by
- 375
- References
- 0
- FWCI
- 4.48
- Type
- journal article
- Language
- en
- Open access
- closed
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- Strazisar, B. R., Anderson, R. R., & White, C. M. (2003). Degradation Pathways for Monoethanolamine in a CO2 Capture Facility. Energy & Fuels. https://doi.org/10.1021/ef020272i
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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