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Bromate Formation during Ozonization of Bromide-Containing Waters: Interaction of Ozone and Hydroxyl Radical Reactions
Open accessAbstract
Kinetic simulations have been tested by laboratory experiments to evaluate the major factors controlling bromate formation during ozonation of waters containing bromide. In the presence of an organic scavenger for OH radicals, bromate formation can be accurately predicted by the molecular ozone mechanism using published reaction rate data, even for waters containing ammonium In the absence of scavengers, OH radical reactions contribute significantly to bromate formation. Carbonate radicals, produced by the oxidation of bicarbonate with OH radicals, oxidize the intermediate hypobromite to bromite, which is further oxidized by ozone to bromate. During drinking water ozonation, molecular ozone controls both the initial oxidation of bromide and the final oxidation of bromite. OH radical reactions contribute to the oxidation of the intermediate oxybromine species. Bromate formation in advanced oxidation processes can be explained by a synergism of ozone and OH radicals.
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Buxton, G. V., Greenstock, C. L., Helman, W. P., & Ross, A. B. (1988) · Journal of Physical and Chemical Reference Data · doi:10.1063/1.555805 · Cited by 12,332
Cited by
von Gunten, U. (2003) · Water Research · doi:10.1016/s0043-1354(02)00458-x · Cited by 1,345
Self-citationZheng, Q., Durkin, D. P., Elenewski, J. E., Sun, Y., Banek, N. A., Hua, L., Chen, H., Wagner, M. J., Zhang, W., & Shuai, D. (2016) · Environmental Science & Technology · doi:10.1021/acs.est.6b02579 · Cited by 328
Remucal, C. K., & Manley, D. (2016) · Environmental Science: Water Research & Technology · doi:10.1039/c6ew00029k · Cited by 214
Synthesis and characterization of CoOx/BiVO4 photocatalysts for the degradation of propyl paraben
Petala, A., Noe, A., Frontistis, Z., Drivas, C., Kennou, S., Mantzavinos, D., & Kondarides, D. I. (2019) · Journal of Hazardous Materials · doi:10.1016/j.jhazmat.2018.03.008 · Cited by 91
Metadata
- Authors
- von Gunten, U., & Hoigne, J.
- Venue
- Environmental Science & Technology
- Publisher
- American Chemical Society (ACS)
- Published
- 1994-07-01
- Volume
- 28
- Issue
- 7
- Pages
- 1234-1242
- ISSN
- 0013-936X (ISSN-L)
- 1520-5851
- OpenAlex
- W2019338346
- Cited by
- 586
- References
- 1
- FWCI
- 16.49
- Type
- journal article
- Language
- en
- Open access
- green
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- von Gunten, U., & Hoigne, J. (1994). Bromate Formation during Ozonization of Bromide-Containing Waters: Interaction of Ozone and Hydroxyl Radical Reactions. Environmental Science & Technology. https://doi.org/10.1021/es00056a009
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